The Raman spectra of the superprotonic conductor Cs5H3(SO4)4·H2O have been investigated in the 300-500 K range. An assignment of bands due to internal and external vibrations in term of approximate type of motions is proposed. The spectroscopic results are used for discussing crystal structures of different phases, the type of structural disorder and phase transitions.
Polarized Raman spectra of Cs5H3(SO4)4· H2O single crystals
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