Low Temperature Structure and Physical Properties of N-Methyl,2,4-Dimethyl Pyridinium (TCNQ)₂

A. Graja Institute of Molecular Physics, Poznan, Poland

M. Przybylski Institute of Molecular Physics, Poznan, Poland

R. Swietlik Institute of Molecular Physics, Poznan, Poland

P. J. Rizkallah Chemistry Department, The University, Nottingham, England

S. C. Wallwork Chemistry Department, The University, Nottingham, England

M. R. Willis Chemistry Department, The University, Nottingham, England

A. Rajchel Institute of Chemistry, A. Mickiewicz, University, Poznan, Poland

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Abstract

The low-temperature (∼ 173 K) structure of NMe2,4MePy(TCNQ)₂ was determined and compared with the room-temperature structure. Electrical, magnetic, dielectric, and spectroscopic properties of the salt are reported. Detailed discussion of the transport properties is presented in terms of a one-electron semiconductor model with low-temperature behaviour controlled by electrically active impurities.

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Low Temperature Structure and Physical Properties of N-Methyl,2,4-Dimethyl Pyridinium (TCNQ)₂

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Low Temperature Structure and Physical Properties of N-Methyl,2,4-Dimethyl Pyridinium (TCNQ)2

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Low Temperature Structure and Physical Properties of N-Methyl,2,4-Dimethyl Pyridinium (TCNQ)₂