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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 37, 1979 - Issue 4
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Original Articles

The electronic structure of the uranyl ion

II. The electronic spectra of CsUO2(NO3)3 and NaUO2(CH3COO)3

R.G. Denning Inorganic Chemistry Laboratory, South Parks Road, Oxford, OX1, 3QR, England
,
D.N.P. Foster Inorganic Chemistry Laboratory, South Parks Road, Oxford, OX1, 3QR, England
,
T.R. Snellgrove Inorganic Chemistry Laboratory, South Parks Road, Oxford, OX1, 3QR, England; Institut für Anorganische Chemie, Freiestrasse 3, CH 3000, Bern 9, Switzerland
&
D.R. Woodwark Inorganic Chemistry Laboratory, South Parks Road, Oxford, OX1, 3QR, England
Pages 1089-1107 | Received 14 Jul 1978, Published online: 23 Aug 2006
 
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Abstract

Polarized single crystal absorption spectra at 4·2 K are reported for CsUO2(NO3)3 and NaUO2(CH3COO)3. Natural and magnetic circular dichroism and Zeeman effect measurements have been made. Measurements have also been made on crystals containing U18O2 2+. In the portion of the spectrum between 21 000 and 30 000 cm-1 seven electronic states have been identified in both CsUO2(NO3)3 and NaUO2(CH3COO)3. In the majority of cases the symmetry of the excited states has been assigned.

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