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Synthetic Communications
An International Journal for Rapid Communication of Synthetic Organic Chemistry
Volume 26, 1996 - Issue 14
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Original Articles

The Michael-Aldol Condensation Approach to the Construction of Key Intermediates in the Synthesis of Nimbolide and Nagilactone A

José A. Bacigaluppo Instituto de Química Orgánica de Síntesis CONICET-Universidad Nacional de Rosario, Facultad de Ciencias Bioquímicas y Farmacéuticas Casilla de Correos, 991, 2000, Rosario, Argentina
,
María I. Colombo Instituto de Química Orgánica de Síntesis CONICET-Universidad Nacional de Rosario, Facultad de Ciencias Bioquímicas y Farmacéuticas Casilla de Correos, 991, 2000, Rosario, Argentina
,
Marcelo D. Preite Instituto de Química Orgánica de Síntesis CONICET-Universidad Nacional de Rosario, Facultad de Ciencias Bioquímicas y Farmacéuticas Casilla de Correos, 991, 2000, Rosario, Argentina
,
Juan Zinczuk Instituto de Química Orgánica de Síntesis CONICET-Universidad Nacional de Rosario, Facultad de Ciencias Bioquímicas y Farmacéuticas Casilla de Correos, 991, 2000, Rosario, Argentina
&
Edmundo A. Rúveda Instituto de Química Orgánica de Síntesis CONICET-Universidad Nacional de Rosario, Facultad de Ciencias Bioquímicas y Farmacéuticas Casilla de Correos, 991, 2000, Rosario, Argentina
Pages 2737-2749 | Received 02 Feb 1996, Published online: 21 Aug 2006
 
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Abstract

A short route for the preparation of highly oxygenated trans-decalines, key intermediates for the synthesis of nimbolide (2a) and nagilactone A (13), by a sequence involving a Michael addition followed by an aldol condensation, is described.

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