Dynamics of the Photoinduced Ionic-to-Neutral Phase Transition in Tetrathiafulvalene- p -chloranil Studied by Femtosecond Time-resolved Reflection Spectroscopy

I. Akimoto Faculty of Systems Engineering, Wakayama University, Sakaedani 930, Wakayama, 640-8510, Japan

K. Tanimura The Institute of Scientific and Industrial Research, Osaka University, Mihogaoka 8-1, Ibaraki, Osaka, 567-0047, Japan

S. Koshihara Department of Materials Science, Tokyo Institute of Technology, Oh-okayama 2-12-1, Megro, Tokyo, 152-8551, Japan

Abstract

Changes in reflection spectra were probed to study the dynamics of photoinduced transformation from ionic to neutral phases in tetrathiafulvalene- p -chloranil crystals. The results have revealed the formation of the precursor of metastable N -phase domains, dynamical lattice relaxation of and proliferation during phase transformation.

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Dynamics of the Photoinduced Ionic-to-Neutral Phase Transition in Tetrathiafulvalene- p -chloranil Studied by Femtosecond Time-resolved Reflection Spectroscopy

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Dynamics of the Photoinduced Ionic-to-Neutral Phase Transition in Tetrathiafulvalene- p -chloranil Studied by Femtosecond Time-resolved Reflection Spectroscopy

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