Abstract
We have observed, in good single crystals of YBa2Cu307-δ, a strong paramagnetic resonance signal characteristic of Cu2+ ions in the | x2 − y2 > state. We observe this signal in both the 40K phase and in the high-Tc ∼ 90K phase. The signal intensity is enhanced at low temperatures, though no anomaly is seen at other temperatures. the signal is broad, with peak to peak width of 0.025 T. Our signal crystals of EuBa2Cu307-δ however, show a resonance that is similar to a Y2BaCu05 phase. This signal intensity is enhanced ∼ 3 times at 77K. There was no significant change in the linewidth with temperature.