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Technical Papers

Significance of Regional Source Contributions to Urban PM-10 Concentrations

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Pages 1286-1291 | Received 19 May 1986, Accepted 04 Aug 1987, Published online: 08 Mar 2012
 

Abstract

Based on data collected in St. Louis, Philadelphia and other eastern U.S. cities, we conclude that a significant fraction of the PM-10 concentration is "background." In these urban areas the background fraction ranges from 35 to 80 percent of the daily, monthly or annual concentration. The bulk of the background appears to be of regional origin. The average chemical makeup of eastern U.S. PM-10 is sulfate as SO4, 21-34 percent; crustal material, 14-39 percent; "unknown" (carbonaceous matter, ammonium, nitrate and water), 36-51 percent, all of which is difficult to apportion to specific sources. Dispersion modeling using a local source inventory can account only for a small portion of the total PM-10 mass. Emission roll-back of local sources may have a limited effect on reducing total concentrations of PM-10.

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