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International Journal of Polymer Analysis and Characterization Volume 21, 2016 - Issue 1
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Original Articles

Characterization of effects of thermal-oxidative aging on styrene-butadiene rubber/silica composites with vitamin C-lanthanum complex

Bangchao ZhongSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, China
,
Zhixin JiaSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, ChinaCorrespondence[email protected]
,
Qifeng ShiSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, China
,
Chao YangSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, China
,
Yuanfang LuoSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, China
&
Demin JiaSchool of Materials Science and Engineering, South China University of Technology, Guangzhou, China
Pages 1-10 | Received 14 Jul 2015, Accepted 21 Jul 2015, Published online: 07 Nov 2015
 
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ABSTRACT

A novel rubber antioxidant, vitamin C-lanthanum complex, was prepared and applied in styrene-butadiene rubber (SBR)/silica composites. The anti-aging behavior of SBR/silica composites with vitamin C-lanthanum complex was systematically investigated by mechanical property retention after aging, oxidation induction time, exothermic enthalpies of thermal oxidation, and thermo-oxidative degradation kinetics. The highlight of this work lies in the fact that several thermal analysis techniques were successfully applied to fully evaluate the thermal-oxidative aging of SBR/silica composites and the vitamin C-lanthanum complex was found to endow SBR/silica composites with better protection against aging than commercial antioxidants, which may be beneficial for better characterization of rubber aging and fruitful for the preparation of highly aging-resistant rubber composites, respectively.

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