Nonlinear Optical Properties of One-Dimensional Platinum Complexes

Takehito Kodzasa National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Toshihide Kamata National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Hirobumi Ushijima National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Hiro Matsuda National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Toshio Fukaya National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Fujio Mizukami National Institute of Materials and Chemical Research, 1-1 Higashi, Tsukuba, 305, JAPAN

Jun Matsunami Department of Chemistry, School of Science and Engineering, Waseda University, Okubo, Shinjuku-ku, Tokyo, 169, JAPAN

Yuji Nagai Department of Chemistry, School of Science and Engineering, Waseda University, Okubo, Shinjuku-ku, Tokyo, 169, JAPAN

Kazuko Matsumoto Department of Chemistry, School of Science and Engineering, Waseda University, Okubo, Shinjuku-ku, Tokyo, 169, JAPAN

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Abstract

Third harmonic generation measurements of composite films of one-dimensional polynuclear platinum complexes with poly(vinyl alcohol) were performed. The third-order nonlinear susceptibility χ⁽³⁾ of the tetranuclear complex was estimated. The χ⁽³⁾ value of the composite film of octanuclear complex was obtained. This value is larger than that of tetranuclear complex. It indicates that the longer platinum chain leads to the enhancement of their third-order optical nonlinearity.

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Nonlinear Optical Properties of One-Dimensional Platinum Complexes

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