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Original Articles

Structural and vibrational properties of a soft-sphere glass: Influence of the quenching rate

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Pages 313-320 | Published online: 13 Aug 2009
 

Abstract

Using classical molecular dynamics simulations combined with the Voronoï tessellation we study, at very low temperatures, the phonon spectrum and the geometrical modifications in a model glass as a function of the quenching rate. The shape of the phonon spectrum is not strongly affected by a decrease in the quenching rate, except for the minimum pulsation ωm, corresponding to the first pseudo-Bragg peak wave-vector, which goes through a marked minimum for the critical quenching rate at which the onset of crystallization is detected by the geometrical analysis. This decrease in ωm can be interpreted as an increase in structural order in the glass phase when the cooling rate is lowered.

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