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Separation Science and Technology Volume 48, 2013 - Issue 9
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Research Article

A New Method for Partitioning of Trivalent Actinides from High-Level Liquid Waste

P. K. NayakFuel Chemistry Group, Indira Gandhi Centre for Atomic Research, Kalpakkam, India
,
R. KumaresanFuel Chemistry Group, Indira Gandhi Centre for Atomic Research, Kalpakkam, India
,
K. A. VenkatesanFuel Chemistry Group, Indira Gandhi Centre for Atomic Research, Kalpakkam, IndiaCorrespondence[email protected]
,
M. P. AntonyFuel Chemistry Group, Indira Gandhi Centre for Atomic Research, Kalpakkam, India
&
P. R. Vasudeva RaoFuel Chemistry Group, Indira Gandhi Centre for Atomic Research, Kalpakkam, India
Pages 1409-1416 | Received 29 Jun 2012, Accepted 03 Oct 2012, Published online: 02 May 2013

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Gabriela A. Picayo, Brian D. Etz, Madeleine A. Eddy, Shubham Vyas & Mark P. Jensen. (2022) Characterization of the ALSEP Process: Investigating Equilibrium and Intermediate Complexes of the Scrub Stage. Solvent Extraction and Ion Exchange 40:6, pages 654-679.
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Yuji Sasaki, Masashi Kaneko, Masahiko Matsumiya, Masahiko Nakase & Kenji Takeshita. (2022) Mutual Separation of Ln and an Using TODGA and DTBA with High Organic Acid Concentrations. Solvent Extraction and Ion Exchange 40:6, pages 620-640.
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А. N. Turanov & V. К. Karandashev. (2018) Synergistic Extraction of U(VI), Th(IV), and Lanthanides(III) from Nitric Acid Solutions Using Mixtures of TODGA and Dinonylnaphthalene Sulfonic Acid. Solvent Extraction and Ion Exchange 36:3, pages 257-271.
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P. K. Nayak, Shivkumar Chaurasia, R. Kumaresan, K. A. Venkatesan, G. G. S. Subramanian, M. P. Antony, P. R. Vasudeva Rao & B. M. Bhanage. (2015) Studies on the Radiochemical Degradation of Tetraethylhexyl Diglycolamide and Ethylhexylphosphoric Acid in n-Dodecane Solution. Separation Science and Technology 50:5, pages 646-653.
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R. S. C. Bose, R. Kumaresan, K. A. Venkatesan, Ramesh L. Gardas, M. P. Antony & P. R. Vasudeva Rao. (2014) Insights Into the Extraction of Am(III) by Aliquat-336 Based Ionic Liquids. Separation Science and Technology 49:15, pages 2338-2345.
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Gregg J. Lumetta, Artem V. Gelis, Jennifer C. Carter, Cynthia M. Niver & Margaret R. Smoot. (2014) The Actinide-Lanthanide Separation Concept. Solvent Extraction and Ion Exchange 32:4, pages 333-347.
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P.K. Nayak, R. Kumaresan, K.A. Venkatesan, M.P. Antony & P.R. Vasudeva Rao. (2014) Extraction Behavior of Am(III) and Eu(III) from Nitric Acid Medium in Tetraoctyldiglycolamide-Bis(2-Ethylhexyl)Phosphoric Acid Solution. Separation Science and Technology 49:8, pages 1186-1191.
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Lei Zhou, Yu Zhou, Caishan Jiao, Meng Zhang, Mingjian He & Yang Gao. (2022) Study of irradiation decomposition products of PUREX solvents on zirconium metal retention behavior. Journal of Radioanalytical and Nuclear Chemistry 332:4, pages 907-916.
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I. V. Kuznetsov, O. N. Budin, A. S. Shchepin, M. Yu. Kalenova, I. M. Mel’nikova, R. V. Saprykin & N. I. Al’zhev. (2022) Annealing of Mineral-Like Host Matrices for High-Level Waste Immobilization. Inorganic Materials 58:6, pages 651-660.
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Gabriela A. Picayo, Brian D. Etz, Shubham Vyas & Mark P. Jensen. (2020) Characterization of the ALSEP Process at Equilibrium: Speciation and Stoichiometry of the Extracted Complex. ACS Omega 5:14, pages 8076-8089.
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K. Rama Swami & K. A. Venkatesan. (2019) Effect of pKa of organophosphorus acidic extractants on the aggregation behavior of diglycolamide in n-dodecane. Journal of Radioanalytical and Nuclear Chemistry 322:2, pages 1055-1064.
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K. Rama swami, T. Prathibha & K.A. Venkatesan. (2019) Aggregation and organic phase splitting behavior of a synergic extractant system probed by dynamic light scattering spectroscopy. Journal of Molecular Liquids 291, pages 111320.
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K. Rama Swami, T. Prathibha, K.A. Venkatesan & M.P. Antony. (2019) Separation of Am(III) from Eu(III) present in 3 M nitric acid medium using completely incinerable binary extractants. Journal of Molecular Liquids 279, pages 427-433.
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A. N. Turanov, V. K. Karandashev & A. N. Yarkevich. (2018) Extraction of REE(III), U(VI), and Th(IV) from Nitric Acid Solutions with Carbamoylmethylphosphine Oxides in the Presence of Dinonylnaphthalenesulfonic Acid. Radiochemistry 60:6, pages 607-612.
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Huiting Yuan, Weixiang Hong, Yushan Zhou, Baisong Pu, Aijun Gong, Tao Xu, Qishan Yang, Fukai Li, Lina Qiu, Weiwei Zhang & Yuning Liu. (2018) Extraction and back-extraction behaviors of 14 rare earth elements from sulfuric acid medium by TODGA. Journal of Rare Earths 36:6, pages 642-647.
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K. Rama Swami, R. Kumaresan, P. K. Nayak, K. A. Venkatesan & M. P. Antony. (2018) Effect of pK a on the extraction behavior of Am(III) in organo phosphorus acid and diglycolamide solvent system . Radiochimica Acta 106:2, pages 107-118.
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K. Rama Swami, R. Kumaresan, K. A. Venkatesan & M. P. Antony. (2018) Minimizing the aggregation of diglycolamide reverse micelles in the n -dodecane phase with bis-(2-ethylhexyl)phosphoric acid “reactive” phase modifier . New Journal of Chemistry 42:11, pages 8891-8899.
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G. Saipriya, R. Kumaresan, P. K. Nayak, K. A. Venkatesan, M. P. Antony & T. Kumar. (2017) Studies on the adsorption behavior of americium and europium on radiolytically degraded solvent impregnated resin containing neutral and acidic extractants. Journal of Radioanalytical and Nuclear Chemistry 314:3, pages 2557-2568.
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K. Rama Swami, R. Kumaresan, P.K. Nayak, K.A. Venkatesan & M.P Antony. (2017) Extraction of Eu(III) in diglycolamide-organophosphorous acid and the interaction of binary solution with Eu(III) studied by FTIR spectroscopy. Vibrational Spectroscopy 93, pages 1-11.
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B. Robert Selvan, K. Dasthaiah, A.S. Suneesh, K.A. Venkatesan, M.P. Antony & R.L. Gardas. (2017) Diglycolic acid modified zirconium phosphate and studies on the extraction of Am(III) and Eu(III) from dilute nitric acid medium. Radiochimica Acta 105:4, pages 275-283.
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K. Rama Swami, R. Kumaresan, K.A. Venkatesan & M.P. Antony. (2017) Synergic extraction of Am(III) and Eu(III) in N,N -dioctyl-2-hydroxyacetamide-bis(2-ethylhexyl)phosphoric acid solvent system. Journal of Molecular Liquids 232, pages 507-515.
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G. Saipriya, R. Kumaresan, P. K. Nayak, K. A. Venkatesan, T. Kumar & M. P. Antony. (2016) Extraction behaviour of Am(III) and Eu(III) from nitric acid medium in TEHDGA-HDEHP impregnated resins. Radiochimica Acta 104:11, pages 781-790.
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S. Rajeswari, M. P. Antony & P. R. Vasudeva Rao. (2015) Evaluation of hydrodynamic suitability of N,N-didodecyl N′,N′-di-octyl diglycolamide: a potential candidate for minor actinide partitioning. Journal of Radioanalytical and Nuclear Chemistry 306:2, pages 407-415.
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Juan Luo, Cong-Zhi Wang, Jian-Hui Lan, Qun-Yan Wu, Yu-Liang Zhao, Zhi-Fang Chai, Chang-Ming Nie & Wei-Qun Shi. (2015) Theoretical studies on the AnO 2 n+ (An = U, Np; n = 1, 2) complexes with di-(2-ethylhexyl)phosphoric acid . Dalton Transactions 44:7, pages 3227-3236.
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Artem V. Gelis & Gregg J. Lumetta. (2014) Actinide Lanthanide Separation Process—ALSEP. Industrial & Engineering Chemistry Research 53:4, pages 1624-1631.
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Hongzhu Chu, Lutao He, Qian Jiang, Yuyu Fang, Yiming Jia, Xiangyang Yuan, Shuliang Zou, Xianghui Li, Wen Feng, Yuanyou Yang, Ning Liu, Shunzhong Luo, Yanqiu Yang, Liang Yang & Lihua Yuan. (2014) CMPO-calix[4]arenes with spacer containing intramolecular hydrogen bonding: Effect of local rigidification on solvent extraction toward f-block elements. Journal of Hazardous Materials 264, pages 211-218.
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Jammu Ravi, K.A. Venkatesan, M.P. Antony, T.G. Srinivasan & P.R. Vasudeva Rao. (2013) Unsymmetrical diglycolamide for the safe management of nuclear waste. Journal of Environmental Chemical Engineering 1:4, pages 690-695.
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