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Solvent Extraction and Ion Exchange Volume 33, 2015 - Issue 3
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Original Articles

Water Soluble PDCA Derivatives for Selective Ln(III)/An(III) and Am(III)/Cm(III) Separation

J. BorriniICSM, Institut de Chimie Séparative de Marcoule, UMR-5257 CNRS/CEA/UM2/ENSCM Bat. 426, Bagnols sur Cèze, France;ICBMS, Institut de Chimie et Biochimie Moléculaire et Supramoléculaire, UMR-5246, Equipe CASYEN, Université de Lyon, Villeurbanne, France;CEA, Nuclear Energy Division, RadioChemistry and Processes Department, SMCS, Elaboration of Separation Processes Laboratory (LEPS), Bagnols sur Cèze, France
,
A. Favre-ReguillonICBMS, Institut de Chimie et Biochimie Moléculaire et Supramoléculaire, UMR-5246, Equipe CASYEN, Université de Lyon, Villeurbanne, France
,
M. LemaireICBMS, Institut de Chimie et Biochimie Moléculaire et Supramoléculaire, UMR-5246, Equipe CASYEN, Université de Lyon, Villeurbanne, France
,
S. GraciaICSM, Institut de Chimie Séparative de Marcoule, UMR-5257 CNRS/CEA/UM2/ENSCM Bat. 426, Bagnols sur Cèze, France
,
G. ArrachartICSM, Institut de Chimie Séparative de Marcoule, UMR-5257 CNRS/CEA/UM2/ENSCM Bat. 426, Bagnols sur Cèze, FranceCorrespondence[email protected]
,
G. BernierCEA, Nuclear Energy Division, RadioChemistry and Processes Department, SMCS, Elaboration of Separation Processes Laboratory (LEPS), Bagnols sur Cèze, France
,
X. HérèsCEA, Nuclear Energy Division, RadioChemistry and Processes Department, SMCS, Elaboration of Separation Processes Laboratory (LEPS), Bagnols sur Cèze, France
,
C. HillCEA, Nuclear Energy Division, RadioChemistry and Processes Department, SMCS, Elaboration of Separation Processes Laboratory (LEPS), Bagnols sur Cèze, France
&
S. Pellet-RostaingICSM, Institut de Chimie Séparative de Marcoule, UMR-5257 CNRS/CEA/UM2/ENSCM Bat. 426, Bagnols sur Cèze, France;ICBMS, Institut de Chimie et Biochimie Moléculaire et Supramoléculaire, UMR-5246, Equipe CASYEN, Université de Lyon, Villeurbanne, FranceCorrespondence[email protected]
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Pages 224-235 | Published online: 02 Dec 2014

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Yufei Wang, Katherine M. Shield & Rebecca J. Abergel. (2023) Hydrophilic Chelators for Aqueous Reprocessing of Spent Nuclear Fuel. Separation & Purification Reviews 0:0, pages 1-19.
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Petr Matveev, Prasanta K. Mohapatra, Stepan N. Kalmykov & Vladimir Petrov. (2021) Solvent extraction systems for mutual separation of Am(III) and Cm(III) from nitric acid solutions. A review of recent state-of-the-art. Solvent Extraction and Ion Exchange 39:7, pages 679-713.
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Andreas Geist, Jean-Marc Adnet, Stéphane Bourg, Christian Ekberg, Hitos Galán, Philippe Guilbaud, Manuel Miguirditchian, Giuseppe Modolo, Chris Rhodes & Robin Taylor. (2021) An overview of solvent extraction processes developed in Europe for advanced nuclear fuel recycling, part 1 — heterogeneous recycling. Separation Science and Technology 56:11, pages 1866-1881.
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Larissa Klaß, Andreas Wilden, Fabian Kreft, Christoph Wagner, Andreas Geist, Petra J. Panak, Irena Herdzik-Koniecko, Jerzy Narbutt & Giuseppe Modolo. (2019) Evaluation of the Hydrophilic Complexant N,N,N’,N’-tetraethyldiglycolamide (TEDGA) and its Methyl-substituted Analogues in the Selective Am(III) Separation. Solvent Extraction and Ion Exchange 37:5, pages 297-312.
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Cécile Marie, Peter Kaufholz, Vincent Vanel, Marie-Thérèse Duchesne, Emilie Russello, Federica Faroldi, Laura Baldini, Alessandro Casnati, Andreas Wilden, Giuseppe Modolo & Manuel Miguirditchian. (2019) Development of a Selective Americium Separation Process Using H4TPAEN as Water-Soluble Stripping Agent. Solvent Extraction and Ion Exchange 37:5, pages 313-327.
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Mark P. Jensen, Renato Chiarizia, Joseph S. Ulicki, Brian D. Spindler, Daniel J. Murphy, M. Mahmun Hossain, Adrián Roca-Sabio, Andrés de Blas & Teresa Rodríguez-Blas. (2015) Solvent Extraction Separation of Trivalent Americium from Curium and the Lanthanides. Solvent Extraction and Ion Exchange 33:4, pages 329-345.
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Articles from other publishers (17)

Marina Amaral Saraiva, Pascal E. Reiller, Cécile Marie & Carole Bresson. (2023) Developing and downscaling a method by HILIC coupled simultaneously to ESIMS and ICPMS to determine the affinity of lanthanide chelating molecules using specific isotope dilution. Journal of Analytical Atomic Spectrometry 38:12, pages 2674-2690.
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Pin-Wen Huang, Cong-Zhi Wang, Qun-Yan Wu, Jian-Hui Lan, Zhi-Fang Chai & Wei-Qun Shi. (2023) Enhanced Am/Eu separation ability of disulfonated diamide N-heterocyclic ligands by adjusting N-, O-donor affinity: A theoretical comparative study. Separation and Purification Technology 319, pages 124030.
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P. Zsabka, A. Wilden, K. Van Hecke, G. Modolo, M. Verwerft & T. Cardinaels. (2023) Beyond U/Pu separation: Separation of americium from the highly active PUREX raffinate. Journal of Nuclear Materials 581, pages 154445.
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V.L. Vidanov, A.Yu. Shadrin, L.I. Tkachenko, E.V. Kenf, P.V. Parabin & S.S. Shirokov. (2021) Separation of americium and curium for transmutation in the fast neutron reactor. Nuclear Engineering and Design 385, pages 111434.
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Petr Distler, Miriam Mindova, Jan Sebesta, Bohumir Gruner, Dmytro Bavol, Richard J. M. Egberink, Willem Verboom, Vasily A. Babain & Jan John. (2021) Stability of Different BTBP and BTPhen Extracting or Masking Compounds against γ Radiation. ACS Omega 6:40, pages 26416-26427.
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Yang Liu, Cong-Zhi Wang, Qun-Yan Wu, Jian-Hui Lan, Zhi-Fang Chai, Qi Liu & Wei-Qun Shi. (2021) Theoretical Insights into Transplutonium Element Separation with Electronically Modulated Phenanthroline-Derived Bis-Triazine Ligands. Inorganic Chemistry 60:14, pages 10267-10279.
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Kathleen Schnaars, Masashi Kaneko & Kiyoshi Fujisawa. (2021) Effect of Oxygen-Donor Charge on Adjacent Nitrogen-Donor Interactions in Eu 3+ Complexes of Mixed N,O-Donor Ligands Demonstrated on a 10-Fold [Eu(TPAMEN)] 3+ Chelate Complex . Inorganic Chemistry 60:4, pages 2477-2491.
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Peter R. Zalupski, Travis S. Grimes, Corey D. Pilgrim, Colt R. Heathman, Santa Jansone-Popova, Katherine R. Johnson, Vyacheslav Bryantsev & Robert C. ChapleskiJrJr. 2021. Including Actinides. Including Actinides 1 162 .
Henning Lumpe, Annika Menke, Christoph Haisch, Peter Mayer, Anke Kabelitz, Kirill V. Yusenko, Ana Guilherme Buzanich, Theresa Block, Rainer Pöttgen, Franziska Emmerling & Lena J. Daumann. (2020) The Earlier the Better: Structural Analysis and Separation of Lanthanides with Pyrroloquinoline Quinone. Chemistry – A European Journal 26:44, pages 10133-10139.
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Pin-Wen Huang, Cong-Zhi Wang, Qun-Yan Wu, Jian-Hui Lan, Zhi-Fang Chai & Wei-Qun Shi. (2020) Quantum chemical studies of selective back-extraction of Am(III) from Eu(III) and Cm(III) with two hydrophilic 1,10-phenanthroline-2,9-bis-triazolyl ligands. Radiochimica Acta 108:7, pages 517-526.
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Jerzy Narbutt. 2020. Liquid-Phase Extraction. Liquid-Phase Extraction 725 744 .
Pin-Wen Huang, Cong-Zhi Wang, Qun-Yan Wu, Jian-Hui Lan, Gang Song, Zhi-Fang Chai & Wei-Qun Shi. (2018) Understanding Am 3+ /Cm 3+ separation with H 4 TPAEN and its hydrophilic derivatives: a quantum chemical study . Physical Chemistry Chemical Physics 20:20, pages 14031-14039.
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Pin-Wen Huang, Cong-Zhi Wang, Qun-Yan Wu, Jian-Hui Lan, Gang Song, Zhi-Fang Chai & Wei-Qun Shi. (2018) Uncovering the impact of ‘capsule’ shaped amine-type ligands on Am( iii )/Eu( iii ) separation . Physical Chemistry Chemical Physics 20:2, pages 1030-1038.
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Nathalie Boubals, Christoph Wagner, Thomas Dumas, Léa Chanèac, Gabriel Manie, Peter Kaufholz, Cécile Marie, Petra J. Panak, Giuseppe Modolo, Andreas Geist & Philippe Guilbaud. (2017) Complexation of Actinide(III) and Lanthanide(III) with H 4 TPAEN for a Separation of Americium from Curium and Lanthanides . Inorganic Chemistry 56:14, pages 7861-7869.
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Andrea Leoncini, Jurriaan Huskens & Willem Verboom. (2017) Ligands for f-element extraction used in the nuclear fuel cycle. Chemical Society Reviews 46:23, pages 7229-7273.
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Łukasz Steczek, Magdalena Rejnis, Jerzy Narbutt, Marie-Christine Charbonnel & Philippe Moisy. (2015) On the stoichiometry and stability of americium(III) complexes with a hydrophilic SO3–Ph–BTP ligand, studied by liquid–liquid extraction. Journal of Radioanalytical and Nuclear Chemistry.
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Stéphanie Gracia, Guilhem Arrachart, Cécile Marie, Simon Chapron, Manuel Miguirditchian & Stéphane Pellet-Rostaing. (2015) Separation of Am (III) by solvent extraction using water-soluble H4tpaen derivatives. Tetrahedron 71:33, pages 5321-5336.
Crossref

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