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Solvent Extraction and Ion Exchange Volume 37, 2019 - Issue 5
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Original Articles

Evaluation of the Hydrophilic Complexant N,N,N’,N’-tetraethyldiglycolamide (TEDGA) and its Methyl-substituted Analogues in the Selective Am(III) Separation

Larissa KlaßForschungszentrum Jülich GmbH (FZJ), Institut für Energie- und Klimaforschung, Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyORCID Iconhttps://orcid.org/0000-0002-3978-0775View further author information
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Andreas WildenForschungszentrum Jülich GmbH (FZJ), Institut für Energie- und Klimaforschung, Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyORCID Iconhttps://orcid.org/0000-0001-5681-3009View further author information
ORCID Icon,
Fabian KreftForschungszentrum Jülich GmbH (FZJ), Institut für Energie- und Klimaforschung, Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyORCID Iconhttps://orcid.org/0000-0002-7475-0686View further author information
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Christoph WagnerInstitute for Nuclear Waste Disposal (INE), Karlsruhe Institute of Technology (KIT), Karlsruhe, GermanyView further author information
,
Andreas GeistInstitute for Nuclear Waste Disposal (INE), Karlsruhe Institute of Technology (KIT), Karlsruhe, GermanyORCID Iconhttps://orcid.org/0000-0003-1436-8247View further author information
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Petra J. PanakInstitute for Nuclear Waste Disposal (INE), Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany;Physikalisch Chemisches Institut (PCI), Ruprecht-Karls-Universität Heidelberg, Heidelberg, GermanyView further author information
,
Irena Herdzik-KonieckoInstitute of Nuclear Chemistry and Technology (ICHTJ), Centre for Radiochemistry and Nuclear Chemistry, Warsaw, PolandORCID Iconhttps://orcid.org/0000-0003-2733-3713View further author information
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Jerzy NarbuttInstitute of Nuclear Chemistry and Technology (ICHTJ), Centre for Radiochemistry and Nuclear Chemistry, Warsaw, PolandORCID Iconhttps://orcid.org/0000-0002-0812-7351View further author information
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Giuseppe ModoloForschungszentrum Jülich GmbH (FZJ), Institut für Energie- und Klimaforschung, Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyCorrespondence[email protected]
ORCID Iconhttps://orcid.org/0000-0001-6490-5595View further author information
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Pages 297-312 | Published online: 27 Aug 2019

Citations (16)

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Read on this site (4)

Yuji Sasaki, Masashi Kaneko, Yasutoshi Ban & Hideya Suzuki. (2023) Mutual separation of Am and Cm using ADAAM (alkyl DiAmide AMine) and reduction of volumes for liquid waste generated via batch-wise multistage extractions. Journal of Nuclear Science and Technology 0:0, pages 1-11.
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Zhibin Liu, Huibo Li, Yaoyang Liu, Chuang Zhao, Caishan Jiao, Yu Zhou, Meng Zhang & Yang Gao. (2022) Recent Progress on the Structure-Performance Relationship between Diglycolamide Extractants and f-Elements. Solvent Extraction and Ion Exchange 40:5, pages 540-570.
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Petr Matveev, Prasanta K. Mohapatra, Stepan N. Kalmykov & Vladimir Petrov. (2021) Solvent extraction systems for mutual separation of Am(III) and Cm(III) from nitric acid solutions. A review of recent state-of-the-art. Solvent Extraction and Ion Exchange 39:7, pages 679-713.
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Manuel Miguirditchian, Vincent Vanel, Cécile Marie, Vincent Pacary, Marie-Christine Charbonnel, Laurence Berthon, Xavier Hérès, Marc Montuir, Christian Sorel, Marie-Jordane Bollesteros, Sylvain Costenoble, Christine Rostaing, Michel Masson & Christophe Poinssot. (2020) Americium Recovery from Highly Active PUREX Raffinate by Solvent Extraction: The EXAm Process. A Review of 10 Years of R&D. Solvent Extraction and Ion Exchange 38:4, pages 365-387.
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Articles from other publishers (12)

Lanlan He, Xueyu Wang, Qiuju Li, Xiao Xiao, Fengfeng Li, Fangxiang Luo, Qingjiang Pan & Songdong Ding. (2023) Novel water-soluble aromatic bisdiglycolamide masking agents for the separation of trivalent americium over lanthanides by NTAamide(n-Oct) extractant. Journal of Environmental Chemical Engineering 11:2, pages 109536.
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Chao Xu, LiYang Zhu, Qian Liu, Suliang Yang, Yun Xue & Guoxin Tian. (2023) A study on the extraction of actinides with a novel carboxylic acid extractant. Journal of Radioanalytical and Nuclear Chemistry 332:4, pages 859-865.
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Patrik Weßling, Michael Trumm, Thomas Sittel, Andreas Geist & Petra J. Panak. (2022) Spectroscopic investigation of the different complexation and extraction properties of diastereomeric diglycolamide ligands. Radiochimica Acta 110:5, pages 291-300.
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Bart Verlinden, Karen Van Hecke, Andreas Wilden, Michelle Hupert, Beatrix Santiago-Schübel, Richard J. M. Egberink, Willem Verboom, Piotr M. Kowalski, Giuseppe Modolo, Marc Verwerft, Koen Binnemans & Thomas Cardinaels. (2022) Gamma radiolytic stability of the novel modified diglycolamide 2,2′-oxybis( N , N -didecylpropanamide) (mTDDGA) for grouped actinide extraction . RSC Advances 12:20, pages 12416-12426.
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Daiki Nomizu, Yuji Sasaki, Masashi Kaneko, Masahiko Matsumiya & Shoichi Katsuta. (2022) Complex formation of light and heavy lanthanides with DGA and DOODA, and its application to mutual separation in DGA–DOODA extraction system. Journal of Radioanalytical and Nuclear Chemistry 331:3, pages 1483-1493.
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Ananda Karak, Bholanath Mahanty, Prasanta K. Mohapatra, Richard J. M. Egberink, Thichur P. Valsala, Darshan B. Sathe, Raj B. Bhatt, Jurriaan Huskens & Willem Verboom. (2021) Highly efficient and selective extraction of Pu(IV) using two alkyl-substituted amides of nitrilo triacetic acid from nitric acid solutions. Separation and Purification Technology 279, pages 119584.
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Ashleigh Kimberlin, Dominique Guillaumont, Sylvie Arpigny, Béatrice Camès, Philippe Guilbaud, Georges Saint-Louis, Hitos Galán & Laurence Berthon. (2021) An experimental and computational look at the radiolytic degradation of TODGA and the effect on metal complexation. New Journal of Chemistry 45:28, pages 12479-12493.
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Masahiko Matsumiya, Yusuke Tsuchida, Yuji Sasaki, Ryoma Ono, Masahiko Nakase & Kenji Takeshita. (2020) Trichotomic separation of light and heavy lanthanides and Am by batchwise multi-stage extractions using TODGA. Journal of Radioanalytical and Nuclear Chemistry 327:1, pages 597-607.
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Andreas Wilden, Fabian Kreft, Dimitri Schneider, Zaina Paparigas, Giuseppe Modolo, Gregg J. Lumetta, Artem V. Gelis, Jack D. Law & Andreas Geist. (2020) Countercurrent Actinide Lanthanide Separation Process (ALSEP) Demonstration Test with a Simulated PUREX Raffinate in Centrifugal Contactors on the Laboratory Scale. Applied Sciences 10:20, pages 7217.
Crossref
T. H. Vu, Jean-Pierre Simonin, A. L. Rollet, R. J. M. Egberink, W. Verboom, M. C. Gullo & A. Casnati. (2020) Liquid/Liquid Extraction Kinetics of Eu(III) and Am(III) by Extractants Designed for the Industrial Reprocessing of Nuclear Wastes. Industrial & Engineering Chemistry Research 59:30, pages 13477-13490.
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Patrik Weßling, Udo Müllich, Elise Guerinoni, Andreas Geist & Petra J. Panak. (2020) Solvent extraction of An(III) and Ln(III) using TODGA in aromatic diluents to suppress third phase formation. Hydrometallurgy 192, pages 105248.
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Gregory P. Horne, Andreas Wilden, Stephen P. Mezyk, Liam Twight, Michelle Hupert, Andrea Stärk, Willem Verboom, Bruce J. Mincher & Giuseppe Modolo. (2019) Gamma radiolysis of hydrophilic diglycolamide ligands in concentrated aqueous nitrate solution. Dalton Transactions 48:45, pages 17005-17013.
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