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Review Articles

Distinctive characteristics of carrier-phonon interactions in optically driven semiconductor quantum dots

ORCID Icon, ORCID Icon &
Article: 1655478 | Received 30 Mar 2019, Accepted 17 Jul 2019, Published online: 09 Sep 2019

Figures & data

Figure 1. Left: Transmission electron microscopy (TEM) picture of a cross section of a single InGaAs QD. Figure by A. Ludwig and J-M. Chauveau [Citation94] © Nature Publishing Group. Center: Calculated phonon spectral density for a spherical QD with a size of 3.8 nm and a flat QD with a lateral size of 5 nm and a height of 1.5 nm. Right: Measured effective phonon spectral density (dots) fitted by a theoretical calculation. The measurements were taken at T=10 K. The inset shows the calculated effective phonon spectral density for different temperatures. The right part is taken from [Citation100] © American Physical Society.

Figure 1. Left: Transmission electron microscopy (TEM) picture of a cross section of a single InGaAs QD. Figure by A. Ludwig and J-M. Chauveau [Citation94] © Nature Publishing Group. Center: Calculated phonon spectral density for a spherical QD with a size of 3.8 nm and a flat QD with a lateral size of 5 nm and a height of 1.5 nm. Right: Measured effective phonon spectral density (dots) fitted by a theoretical calculation. The measurements were taken at T=10 K. The inset shows the calculated effective phonon spectral density for different temperatures. The right part is taken from [Citation100] © American Physical Society.

Figure 2. Left: Calculated normalized emission spectrum from a single QD at different temperatures. Note the logarithmic scale. Inset: fraction of the intensity in the sidebands. Taken from Ref [Citation163]. © American Physical Society. Right: Calculated spectrum from a QD in a photonic cavity (red dotted line) and without cavity (black line). The cavity spectrum is indicated by the blue, dashed line. Note the logarithmic scale. Taken from Ref [Citation168]. © American Physical Society.

Figure 2. Left: Calculated normalized emission spectrum from a single QD at different temperatures. Note the logarithmic scale. Inset: fraction of the intensity in the sidebands. Taken from Ref [Citation163]. © American Physical Society. Right: Calculated spectrum from a QD in a photonic cavity (red dotted line) and without cavity (black line). The cavity spectrum is indicated by the blue, dashed line. Note the logarithmic scale. Taken from Ref [Citation168]. © American Physical Society.

Figure 3. Top: Exciton occupation in a two-level QD coupled to phonons as a function of time and excitation strength for a continuous excitation with the Rabi frequency ΩR switched on instantaneously at t=0. Bottom: Normalized phonon displacement u˜ at a sphere outside the QD. The dashed lines mark the resonance with the maximum of the phonon spectral density. Results adopted from [Citation118]  © IOP Publishing. Right: Dynamics of the Bloch vector on the Bloch sphere for the phonon-damped Rabi oscillations.

Figure 3. Top: Exciton occupation in a two-level QD coupled to phonons as a function of time and excitation strength for a continuous excitation with the Rabi frequency ΩR switched on instantaneously at t=0. Bottom: Normalized phonon displacement u˜ at a sphere outside the QD. The dashed lines mark the resonance with the maximum of the phonon spectral density. Results adopted from [Citation118]  © IOP Publishing. Right: Dynamics of the Bloch vector on the Bloch sphere for the phonon-damped Rabi oscillations.

Figure 4. (a) Experimentally measured fluorescence and (b) theoretically calculated occupation corresponding to the excited state of a QD driven by a chirped laser pulse with different chirp rates as indicated. Taken from [Citation206] © American Physical Society.

Figure 4. (a) Experimentally measured fluorescence and (b) theoretically calculated occupation corresponding to the excited state of a QD driven by a chirped laser pulse with different chirp rates as indicated. Taken from [Citation206] © American Physical Society.

Figure 5. Left: Phonon-assisted state preparation using two-photon excitation (TPE) for different laser detunings and two excitation strength 1π and 7π. Dots are experimental data, while the solid lines are fits. Taken from [Citation218] under a Creative Commons Attribution. Right: Dynamics of the Bloch vector for phonon-assisted state preparation with (a,b) dynamics of the Bloch sphere and (c,d) length of the Bloch vector for excitation with a Gaussian pulse (a,c) and with a rectangular pulse with either a smooth switch on (blue) or off (red) (b,d). Taken from [Citation202]  © American Physical Society.

Figure 5. Left: Phonon-assisted state preparation using two-photon excitation (TPE) for different laser detunings and two excitation strength 1π and 7π. Dots are experimental data, while the solid lines are fits. Taken from [Citation218] under a Creative Commons Attribution. Right: Dynamics of the Bloch vector for phonon-assisted state preparation with (a,b) dynamics of the Bloch sphere and (c,d) length of the Bloch vector for excitation with a Gaussian pulse (a,c) and with a rectangular pulse with either a smooth switch on (blue) or off (red) (b,d). Taken from [Citation202]  © American Physical Society.

Figure 6. Impact of the temperature on the two-photon interference (TPI) visibility. (a)-(c) TPI histograms for co-polarized configuration at 10, 25, and 35 K and corresponding fits (red solid curves). (d) Experimentally obtained TPI visibilities for various temperatures together with theoretical results accounting for two stochastic forces. Taken from Ref [Citation257]. © American Physical Society.

Figure 6. Impact of the temperature on the two-photon interference (TPI) visibility. (a)-(c) TPI histograms for co-polarized configuration at 10, 25, and 35 K and corresponding fits (red solid curves). (d) Experimentally obtained TPI visibilities for various temperatures together with theoretical results accounting for two stochastic forces. Taken from Ref [Citation257]. © American Physical Society.

Figure 7. Brightness B (panels a, b) and single-photon purity P (panels c, d) as a function of the excitation pulse area θ of a pulse in the pulse train for selected laser-exciton detunings ΔωLX. The left column (a, c) is the result of a phonon-free calculation, the right column (b, d) includes the coupling to a continuum of LA phonons. The purity curves have been cut off at the lower end at 50% in order to highlight the behavior at elevated P values. Results are taken from [Citation288].

Figure 7. Brightness B (panels a, b) and single-photon purity P (panels c, d) as a function of the excitation pulse area θ of a pulse in the pulse train for selected laser-exciton detunings ΔωLX. The left column (a, c) is the result of a phonon-free calculation, the right column (b, d) includes the coupling to a continuum of LA phonons. The purity curves have been cut off at the lower end at 50% in order to highlight the behavior at elevated P values. Results are taken from [Citation288].

Figure 8. Cavity photon distribution at t = 3 ns for different detunings δ and a cavity coupling g=0.1 meV equal to the laser driving strength. (a) without dot-phonon interaction and (b) with phonons at temperature T = 4 K. (c) Photon distribution at detuning δ=18μeV with phonons at T = 4 K compared with Poissonian and thermal distributions. Figure taken from [Citation37] © American Physical Society.

Figure 8. Cavity photon distribution at t = 3 ns for different detunings δ and a cavity coupling ℏg=0.1 meV equal to the laser driving strength. (a) without dot-phonon interaction and (b) with phonons at temperature T = 4 K. (c) Photon distribution at detuning δ=−18μeV with phonons at T = 4 K compared with Poissonian and thermal distributions. Figure taken from [Citation37] © American Physical Society.