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The Journal of Adhesion Volume 97, 2021 - Issue 4
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Research Article

Enhanced adhesion property of aramid fibers by polyphenol-metal iron complexation and silane grafting

Lei Wanga AECC Beijing Institute of Aeronautical Materials (BIAM), Beijing, P. R. China;b State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. ChinaView further author information
,
Bo Zhangb State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. China;c Ministry of Education, Engineering Research Center of Elastomer Materials on Energy Conservation and Resources, Beijing, P. R. ChinaView further author information
,
Xue Lib State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. China;c Ministry of Education, Engineering Research Center of Elastomer Materials on Energy Conservation and Resources, Beijing, P. R. ChinaView further author information
,
Wencai Wangb State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. China;c Ministry of Education, Engineering Research Center of Elastomer Materials on Energy Conservation and Resources, Beijing, P. R. ChinaCorrespondence[email protected]
View further author information
,
Ming Tianb State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. China;c Ministry of Education, Engineering Research Center of Elastomer Materials on Energy Conservation and Resources, Beijing, P. R. ChinaView further author information
,
Zhaodong Fana AECC Beijing Institute of Aeronautical Materials (BIAM), Beijing, P. R. ChinaCorrespondence[email protected]
View further author information
&
Liqun Zhangb State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, P. R. China;c Ministry of Education, Engineering Research Center of Elastomer Materials on Energy Conservation and Resources, Beijing, P. R. ChinaView further author information
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Pages 346-360 | Received 25 Jun 2019, Accepted 08 Sep 2019, Published online: 16 Sep 2019
 
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ABSTRACT

In this work, a green and efficient method for the surface modification of aramid fibers is proposed, aiming to enhance their adhesion property with rubber matrix. The surface of the aramid fibers was pre-deposited with a polyphenol-metal complex coating via rapid (1 min) complexation between FeIII ions and tannic acid (TA), followed by silane grafting. The influences of reactant concentration and reaction temperature on the grafting efficiency of bis-(γ-triethoxysilylpropyl)-tetrasulfide (Si69) were also characterized. The adhesion force of the modified aramid fibers/rubber composites showed a maximum improvement of 73.6% compared to that of untreated aramid fibers/rubber composites. This approach showed great potential in rubber industry due to its low-cost and high-efficiency.

Conflict of interest statement

The authors declare no competing financial interest.

Supplementary material

The supplemental data for this article can be accessed at here.

Additional information

Funding

This work was supported by the National Natural Science Foundation of China [NO. 51373010 and NO. 51521062].

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