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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 101, 2003 - Issue 3
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Original Articles

Polarization components of rototranslational light scattering spectra from gaseous SF6

K. NOWICKA Nonlinear Optics Division, Institute of Physics, Adam Mickiewicz University, Umultowska 85, 61-614, Poznan, Poland
,
T. BANCEWICZ Nonlinear Optics Division, Institute of Physics, Adam Mickiewicz University, Umultowska 85, 61-614, Poznan, Poland
,
J.-L. GODET Laboratoire des Propriétiés Optiques des Matériaux et Applications, Université d'Angers, 2 boulevard Lavoisier, 49045, Angers, France
,
Y. LE DUFF Laboratoire des Propriétiés Optiques des Matériaux et Applications, Université d'Angers, 2 boulevard Lavoisier, 49045, Angers, France
&
F. RACHET Laboratoire des Propriétiés Optiques des Matériaux et Applications, Université d'Angers, 2 boulevard Lavoisier, 49045, Angers, France
Pages 389-396 | Received 04 Jul 2002, Accepted 19 Sep 2002, Published online: 18 Nov 2009
 
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Abstract

Experimental binary anisotropic and isotropic collision-induced scattering spectra of gaseous sulphur hexafluoride at room temperature are reported on an absolute scale up to 210cm-1. On the basis of a comparison of experiment with theoretical computations of scattering intensities, the value of the independent component E of the dipole-octopole polarizability tensor is discussed for several intermolecular potentials and compared with a recent ab initio theoretical value. A recommended value of E is given.

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