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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 115, 2017 - Issue 9-12: Special Issue in Honour of Professor Johann Fischer
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Articles

Virial coefficients of the additive hard-sphere binary mixtures up to the eighth

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Pages 1051-1056 | Received 27 Jun 2016, Accepted 12 Aug 2016, Published online: 08 Sep 2016
 

ABSTRACT

The fifth to eighth virial coefficients of the additive hard-sphere binary mixtures are accurately calculated in the whole range of sphere diameter ratios. Calculations are based on an extension of the technique for topological analysis of the Ree–Hoover diagrams and the standard Metropolis Monte Carlo algorithm. The results for the fifth to the seventh partial virial coefficients are compared with literature data. The eighth virial coefficients are new. The results are also compared with a semi-empirical analytical equation due to Wheatley and discussed.

Disclosure statement

No potential conflict of interest was reported by the authors.

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