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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 29, 1975 - Issue 3
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Original Articles

Vibronic borrowing of angular momentum in the 1B2u state of benzene

I.N. Douglas School of Chemical Sciences, University of East Anglia, Norwich, NOR 88C; Department of Solid State Physics, Research School of Physical Sciences, The Australian National University, Canberra, A.C.T., 2600, Australia
,
R. Grinter School of Chemical Sciences, University of East Anglia, Norwich, NOR 88C
&
A.J. Thomson School of Chemical Sciences, University of East Anglia, Norwich, NOR 88C
Pages 673-679 | Received 05 Aug 1974, Published online: 22 Aug 2006
 
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Abstract

The origin of the positive A term in the magnetic circular dichroism spectrum of the A 0 0 band of the 1 B 2u ← 1 A 1g transition of benzene in the vapour phase is investigated. The appearance of this A term is shown to be consistent with the vibronic borrowing of angular momentum from the allowed 1 E 1u ← 1 A 1g transition for which a positive A term has also been observed. Comparison is made with a calculation of the A term in the 1 B 1u ← 1 A 1g transition of benzene.

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