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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 49, 1983 - Issue 1
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Original Articles

Line displacement and line width in the binary collision theory of the vibrational phase relaxation

R. Ouillon Département de Recherches Physiques, Laboratoire associé au C.N.R.S., Université Pierre et Marie Curie, No. 71, Tour 22, 4, place Jussieu, 75230, Paris Cedex, France
,
V. Sergiescu Faculté des Sciences d'Angers, Laboratoire d'Optique des Fluides, 2, boulevard Lavoisier, 49045, Angers Cedex, France
&
R. Tascón D'León Département de Recherches Physiques, Laboratoire associé au C.N.R.S., Université Pierre et Marie Curie, No. 71, Tour 22, 4, place Jussieu, 75230, Paris Cedex, France
Pages 151-158 | Received 29 Oct 1982, Accepted 08 Jan 1983, Published online: 23 Aug 2006
 
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Abstract

We present an elementary kinetic calculation of the displacement and width of a Raman line due to vibrational phase relaxation. The binary collision model is used and the relation between the two effects is stressed. The calculated values are compared with the experimental ones for gaseous (H2/H2, H2/He, H2/Ar) and liquid (H2/SF6, N2O/SF6, N2O/CCl4) systems. A repulsive potential is used.

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