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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 72, 1991 - Issue 2
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Original Articles

Three-body correlation spectra from collision-induced light scattering by SF6 and CF4

S.M. El-Sheikh Department of Physics, University of Manitoba, Winnipeg, Manitoba, Canada, R3T 2N2
,
G.C. Tabisz Department of Physics, University of Manitoba, Winnipeg, Manitoba, Canada, R3T 2N2
&
L. Ulivi Istituto di Elettronica Quantistica del CNR, Via Panciatichi 56/30, 50127, Firenze, Italy
Pages 345-352 | Received 23 Mar 1990, Accepted 25 Jun 1990, Published online: 22 Aug 2006
 
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Abstract

New data on the three-body correlation spectra obtained from collision-induced light scattering by SF6 and CF4 at 295 K are reported. The experimental zeroth and second moments are compared with calculations based on a pairwise-additive triplet cluster polarizability. Dipole-induced-dipole and electron-overlap contributions to the pair polarizabilities are considered. Comments are made on the adequacy of existing potentials for describing the scattering.

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