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Phosphorus, Sulfur, and Silicon and the Related Elements Volume 186, 2011 - Issue 4: 18th International Conference on Phosphorus Chemistry (ICPC2010)
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I. Synthesis and Applications in Catalysis

Diverse Reactions of Sterically Protected 1,3-Diphosphacyclobutane-2,4-diyls with Hydride

Shigekazu Ito Department of Applied Chemistry, Graduate School of Science and Engineering, Tokyo Institute of Technology, Ookayama, Tokyo, Japan
,
Joji Miura Department of Chemistry, Graduate School of Science, Tohoku University, Sendai, Japan
,
Noboru Morita Department of Chemistry, Graduate School of Science, Tohoku University, Sendai, Japan
,
Masaaki Yoshifuji Department of Chemistry, The University of Alabama, Tuscaloosa, Alabama, USA
&
Anthony J. Arduengo III Department of Chemistry, The University of Alabama, Tuscaloosa, Alabama, USA
Pages 756-757 | Received 28 Jul 2010, Accepted 19 Aug 2010, Published online: 25 Apr 2011
 
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Abstract

Stable 1,3-diphosphacyclobutane-2,4-diyls carrying a substituent such as benzyl moiety react with hydride to cause reductive P–C bond cleavage leading to the cyclic phosphaallyl anion, which is the synthetic intermediate of biradicals.

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