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Phosphorus, Sulfur, and Silicon and the Related Elements Volume 190, 2015 - Issue 7
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Original Articles

Mild, Selective, and Efficient Oxidation of Sulfides to Sulfoxides Catalyzed by Mn(Iii)-Salen Complexes

Alessandro BismutoDipartimento di Scienze Chimiche, Università di Napoli “Federico II”, Complesso Universitario Monte S. Angelo, Via Cintia, I-80126, Napoli, Italy
,
Maria E. CucciolitoDipartimento di Scienze Chimiche, Università di Napoli “Federico II”, Complesso Universitario Monte S. Angelo, Via Cintia, I-80126, Napoli, Italy;Consorzio Interuniversitario di Reattività Chimica e Catalisi, via Celso Ulpiani 27 70126, Bari, Italy
,
Francesco RuffoDipartimento di Scienze Chimiche, Università di Napoli “Federico II”, Complesso Universitario Monte S. Angelo, Via Cintia, I-80126, Napoli, Italy;Consorzio Interuniversitario di Reattività Chimica e Catalisi, via Celso Ulpiani 27 70126, Bari, ItalyCorrespondence[email protected]
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Aldo VitaglianoDipartimento di Scienze Chimiche, Università di Napoli “Federico II”, Complesso Universitario Monte S. Angelo, Via Cintia, I-80126, Napoli, Italy;Consorzio Interuniversitario di Reattività Chimica e Catalisi, via Celso Ulpiani 27 70126, Bari, Italy
&
Massimiliano CurcioInstitute for Polymers, Composites and Biomaterials (IPCB), National Research Council of Italy (CNR), P.le Fermi 1, I-80055Portici, Napoli, Italy
Pages 1021-1028 | Received 03 Jul 2014, Accepted 02 Aug 2014, Published online: 25 Jul 2015
 
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GRAPHICAL ABSTRACT

Abstract

A detailed optimization of the catalytic environment for the oxidation of sulfides promoted by Mn(salen)/H2O2 systems is proposed. The experimental setup is demonstrated to be active towards different substrates, providing TOFs up to 9300 h−1, which are among the highest reported for homogeneous catalysts employed in sulfoxidation reactions.

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