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Energy Sources, Part A: Recovery, Utilization, and Environmental Effects Volume 32, 2010 - Issue 15
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Original Articles

The Effect of Co Loading on the Performance of CoxMn0.06/SiO2 Catalysts for the Synthesis of Light Hydrocarbons from CO Hydrogenation

J.-J. Zhao Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China; Department of Science, Bengbu College, Bengbu, Anhui, China
,
Z.-M. Zong Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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J.-J. Li Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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H.-S. Xie Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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T. Liu Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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Z.-S. Yao Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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Y. Huang Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
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X.-Y. Wei Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China; Hubei Coal Conversion and New Carbon Materials Laboratory, Wuhan University of Science and Technology, Wuhan, Hubei, China
&
W.-J. Zhao Key Laboratory of Coal Processing and Efficient Utilization (Ministry of Education), School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu, China
 show all
Pages 1408-1415 | Received 16 Nov 2008, Accepted 21 Dec 2008, Published online: 07 Jun 2010
 
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Abstract

A series of CoxMn0.06/SiO2 catalysts, which were used for the synthesis of light hydrocarbons from CO hydrogenation, were prepared. The effects of reaction temperature, the morphological and structural properties of the catalysts on the CO conversion and product selectivity were examined. The results show that both CO conversion and C2 to C4 hydrocarbon selectivity are significantly affected by the amount of Co loaded onto the catalysts. The optimum Co content was determined to be 10 wt% (i.e., for Co0.10Mn0.06/SiO2) catalyst, and corresponding CO conversion and the selectivity to C2 to C4 hydrocarbons are 95.3 and 80.6%, respectively, at 400°C.

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