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REVIEW

Reassessment of Reactor Coolant and Iodine Chemistry under Accident Conditions

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Pages 1023-1031 | Received 11 Mar 2009, Accepted 03 Aug 2009, Published online: 05 Jan 2012

References

  • U.S. NRC . 1975 . Reactor Safety Study: An Assessment of Accident Risks in U.S. Commercial Nuclear Power Plants , WASH-1400 (NUREG 75/014)
  • Kemney , J. G. , Babbitt , B. , Haggetry , P. E. , Lewis , C. , Marks , P. A. , Marrett , C. B. , McBride , L. , McPerson , H. C. , Peterson , R. W. , Pigford , T. H. , Tatlor , T. B. and Trunk , A. D. 1979 . Report on the President's Commission on the Accident at Three Mile Island New York : Pergamon Press, inc .
  • Lemire , R. J. , Paquette , J. , Torgerson , D. F. , Wren , D. J. and Fletcher , J. W. 1981 . Assessment of Iodine Behavior in Reactor Containment Buildings from a Chemical Perspective , AECL-6812 AECL .
  • Deanne , M. and Pottter , P. E. , eds. 1985 . Proc. Specialists Workshop on Iodine Chemistry in Reactor Safety Harwell, England : AERE . Sep. 11–12, 1985
  • Bell , J. T. , Campbell , D. O. , Lietzke , M. H. , Palmer , D. A. and Toth , L. M. 1982 . Aqueous Iodine Chemistry in LWR Accidents: Review and Assessement , NUREG/CR-2493, ORNL-5824
  • Niemczyk , S. J. , ed. 1987 . Proc. Symposium on Chemical Phenomena Associated with Radioactivity Releases During Severe Nuclear Plant Accidents Anaheim, California , , USA Sep. 9–12, 1986, NUREG/CR-0078
  • Beahm , E. C. , Shockley , W. E. , Weber , C. F. , Wisbey , S. J. and Wang , Y. M. 1986 . Chemistry and Transport of Iodine in Containment , NUREG/CR-4697
  • Ishigure , K. , Saeki , M. , Soda , K. and Sugimoto , J. , eds. 1991 . Proc. The Third CSNI Workshop on Iodine Chemistry in Reactor Safety, Tokai-mura, Japan, Sep. 11–13 92 – 012 . NEA/CSNI/R(91)15, JAERI-M, 1992
  • McFarlane , J. , Wren , J. C. and Lemire , R. J. 2002 . “Chemical speciation of iodine source term to containment” . Nucl. Technol. , 138 : 162 – 178 .
  • Cantrel , L. 2006 . “Radiochemistry of iodine: Outcomes of the CAIMAN program” . Nucl. Technol. , 156 ( 1 ) : 11 – 28 .
  • Clement , B. , Hanniet-Girault , N. , Repetto , G. , Jacquemain , D. , Jones , A. V. , Kissane , M. P. and van der Hardt , P. 2003 . “LWR severe accident simulation: Synthesis of results and interpretation of the first Phebus FP experiment FPTO” . Nucl. Eng. Des. , 226 ( 1 ) : 5 – 82 .
  • Mueller , K. 2008 . “Validation of severe accident codes on the PHEBUS fission product tests in the framework of the PHEBEN-2 project” . Nucl. Technol. , 163 : 209 – 227 .
  • Soffer , L. , Burson , S. B. , Ferrell , C. M. , Lee , R. Y. and Ridgely , J. N. 1995 . Accident Source Terms for Light-Water Nuclear Power Plants , NUREG-1465
  • U.S. AEC . 1974 . Assumptions Used for Evaluating the Potential Radiological Consequences of a Loss of Coolant Accident for Boiling Water Reactors , Regulatory Guide 1.3 Revision 2
  • U.S. AEC . 1974 . Assumptions Used for Evaluating the Potential Radiological Consequences of a Loss of Coolant Accident for Pressurized Water Reactors , Regulatory Guide 1.4 Revision 2
  • U.S. NRC . 2004 . The United States of America Third National Report for the Convention on Nuclear Safety , NUREG-1650 Rev.1
  • Lin , C. C. 1981 . Anticipated Chemical Behavior of Iodine under LOCA Conditions , NEDO-25370, Class I General Electric Company .
  • Careway , M. A. 1980 . Calculation of Fission Product Inventory and Spectra—RADC101 Program , NEDO-25176
  • EPRI . 2003 . Pressurized Water Reactor Primary Water Chemistry Guidelines: Volume 1 , Revision 5, EPRI Palo Alto , CA 1002884
  • Lin , C. C. 2000 . “Hydrogen water chemistry technology in boiling water reactors” . Nucl. Technol. , 130 ( 1 ) : 59 – 70 .
  • Wren , J. C. , Ball , J. M. and Glowa , G. A. 2000 . “The chemistry of iodine in containment” . Nucl. Technol. , 129 : 297 – 325 .
  • Beahm , E. C. , Weber , C. F. , Hress , T. S. and Parker , G. W. 1992 . Iodine Chemical Forms in LWR Sever Accidents, Final Report, NUREG/CR-5732
  • Bell , J. T. , Lietzke , M. H. and Palmer , D. A. 1982 . Predicted Rates of Formation of Iodine Hydrolysis Species at pH Levels, Concentrations, and Temperatures Anticipated in LWR Accidents , NUREG/CR-2900
  • Weber , C. F. , Beahm , E. C. and Kress , T. S. 1992 . Models of Iodine Behavior in Reactor Containments , ORNL/TM-12202
  • Haimovic , O. and Treinin , A. 1967 . “Disproportionation of hypoiodite” . J. Phys. Chem. , 71 ( 6 ) : 1941
  • Lin , C. C. 1981 . “Volatility of iodine in dilute aqueous solutions” . J. Inorg. Nucl. Chem. , 43 ( 12 ) : 3229 – 3238 .
  • Lin , C. C. 1980 . “Chemical effects of gamma radiation on iodine in aqueous solutions” . J. Inorg. Nucl. Chem. , 42 ( 8 ) : 1101 – 1107 .
  • Ishigure , K. , Shiraishi , H. and Okuda , H. 1988 . “Radiation chemistry of aqueous iodine systems under nuclear reactor accident conditions” . Radiat. Phys. Chem. , 32 ( 4 ) : 593 – 597 .
  • Naritomi , M. , Nagai , N. , Okagawa , S. and Ishiwatari , N. 1991 . “Batchtype tests on formations of volatile iodine species from aqueous iodide solution under 60Co γ-ray irradiation” . In Proc. The Third CSNI Workshop on Iodine Chemistry in Reactor Safety, Tokai-mura, Japan, Sep. 11–13 97 1992
  • Lin , C. C. , Wang , C. F. , Sun , Y. C. , Chao , J. H. and Tseng , C. L. 2006 . “Radiation effects on gaseous iodine at very low concentrations” . J. Radioanal. Nucl. Chem. , 268 ( 2 ) : 419 – 426 .
  • Postma , E. and Zavodoski , R. W. 1972 . Review of Organic Iodide Formation under Accident Conditions in Water-Cooled Reactors , WASH-1233
  • Beahm , E. C. , Shockley , W. E. and Culberson , O. L. 1985 . Organic Iodide Formation Following Nuclear Reactor Accidents , NUREG/CR-4327
  • Zoulalian , A. and Belval-Haltier , E. 2000 . “Interaction between molecular iodine in a gas phase and paints aged in a nuclear power plant” . Nucl. Technol. , 130 : 362 – 371 .
  • Wren , J. C. , Ball , J. M. and Glowa , G. A. 1999 . “The interaction of iodine with organic material in containment” . Nucl. Technol. , 125 : 337 – 362 .
  • Wisbey , S. J. , Beahm , E. C. , Shockley , W. E. and Wang , Y. M. 1987 . “Iodine behavior in containment under accident conditions” . In Proc. Symposium on Chemical Phenomena Associated with Redioactivity Releases During Severe Nuclear Plant Accidents 6 – 29 . Anaheim, California , , USA Sep. 9–12, 1986
  • Guentay , S. , Cripps , R. , Jaeckel , B. and Bruchertseifer , H. 2007 . “Radiochemical studies of the retention of volatile iodine in aqueous solutions” . J. Radioanal. Nucl. Chem. , 273 : 557 – 561 .
  • Moelwyn-Hughes , E. A. 1953 . “The kinetics of hydrolysis” . Proc. Roy. Soc. , 220 : 386
  • Heppolette , R. L. and Robertson , R. E. 1959 . “The neutral hydrolysis of the methyl hadides” . Proc. Roy. Soc. , 252 : 273
  • Adachi , M. , Eguchi , W. and Maoka , T. 1974 . J. Chem. Eng. , 7 : 364
  • Glowa , G. A. and Wren , J. C. 2003 . “Aqueous-gas phase partitioning and hydrolysis of organic iodides” . Can. J. Chem. , 81 : 230 – 243 .
  • Nishizawa , Y. , Kigoshi , Y. , Oshima , S. , Ozawa , Y. and Malkawa , T. 1969 . “Gas-water partition coefficient of iodine and organic iodides” . J. At. Energy Soc. Jpn. , 11 : 205
  • Parsly , L. H. 1970 . Design Conditions of Reactor Containment—Part IV. Calculations of Iodine-Water Partition Coefficients , ORNL/TM-2412
  • Toth , L. M. , Pannel , K. D. and Kirkland , O. L. 1984 . The Chemical Behavior of Iodine in Aqueous Solutions up to 150°C , NUREG/CR-3514
  • Furrer , M. , Cripps , R. C. and Gubler , R. 1985 . “Measurement of the iodine partition coefficient” . Nucl. Technol. , 70 ( 2 ) : 290 – 293 .
  • Gwyther , J. R. and Turner , D. J. 1989 . Volatility of Hypoiodic Acid in Steam, Water Chemistry of Nuclear Reactor System 5 , BNES Vol. 1 , 289
  • Beahm , E. C. , Daish , S. R. , Shockley , W. E. and Hopenfeld , J. 1990 . “Iodine partitioning in pressurized water reactor steam generator accidents” . Nucl. Technol. , 90 ( 1 ) : 16 – 22 .
  • Pelletier , C. A. and Hemphill , R. T. 1979 . Nuclear Power Plant Related Iodine Partition Coefficients , EPRI NP-1271
  • Kelly , J. L. , Muler , R. U. and Babad , C. J. 1985 . “Experimental investigation of the iodine partition coefficient” . Nucl. Technol. , 71 : 426 – 429 .
  • Evans , G. J. , Jervis , R. E. and Csillag , E. G. 1988 . “The air/water partitioning of radioiodine: An experimental assessment” . J. Radioanal. Nucl. Chem. , 124 : 145 – 155 .
  • Marshall , P. W. , Lutz , J. B. and Kelly , J. L. 1987 . “Gamma radiation effects on time-dependent iodine partitioning” . Nucl. Technol. , 76 ( 3 ) : 400 – 407 .
  • Evans , G. J. 1996 . “Measurement and modeling of iodine volatility above irradiated CsI solutions” . Nucl. Technol. , 116 ( 3 ) : 293 – 305 .
  • Lutz , J. B. and Kelly , J. L. 1988 . “The effects of organic impurities on the partitioning of iodine” . Nucl. Technol. , 80 ( 3 ) : 431 – 442 .
  • Allen , T. L. and Keeffer , M. R. 1955 . “The formation of hypoiodous and hydrated iodine cation by the hydrolysis of indine” . J. Am. Chem. Soc. , 77 : 2957 – 2960 .
  • Dickinson , S. and Sims , H. E. 2000 . “Development of the INSPECT model for the prediction of iodine volatility from irradiated solution” . Nucl. Technol. , 129 ( 3 ) : 374 – 386 .
  • Lin , C. C. 1983 . “Chemical behavior and distribution of volatile radionuclides in a BWR system with forward-pumped heater drains” . In Proc. Int. Conf. Water Chemistry of Nuclear Reactor Systems 3 103 BNES, London
  • Lin , C. C. 1992 . “Chemical behavior of radioiodine in boiling water reactor systems 2. Effects of hydrogen water chemistry” . Nucl. Technol. , 97 ( 1 ) : 71 – 78 .
  • Guentay , S. , Cripps , R. C. , Jackel , B. and Bruchertseifer , H. 2005 . “Iodine behavior during a severe accident in a nuclear power plant” . Chimia , 59 ( 12 ) : 957 – 965 .
  • Cline , J. M. 1981 . Measurement of 129 I and Radioactive Particulate Concentrations in the TMI-2 Containment Atmosphere During and After the Venting , GEND-009
  • Volleque , P. G. 1979 . Iodine Species in Reactor Effluents and in the Environment , EPRI NP-1269
  • Pelletier , C. A. 1973 . Result of Indepent Measurements of Radioactivity in Process System and Effluents of Boiling Water Reactors Environmental Protection Branch USAEC .
  • Lin , C. C. 1973 . The Behavior of Radioiodine in BWR Systems, A Study at Nime Mile Point , NEDM-12446
  • Potter , E. C. and Mann , G. M. W. 1965 . “The fast linear growth of magnetite on mild steel in high-temperature aqueous conditions” . Br. Corros. J. , 1 ( 1 ) : 26
  • Lin , C. C. 1973 . Behavior of Carrier-free Iodine: The Formation of Volatile Organic Iodine , NEDM-12452
  • Saeki , M. and Tachikawa , E. 1997 . J. Atom. Energy Soc. Jpn. , 19 : 332
  • Nakashima , M. , Saeki , M. , Aratono , Y. and Tachikawa , E. 1981 . “Release of radioindine from UO2 during reactor operation” . Int. J. Appl. Radiat. Isot. , 32 ( 6 ) : 397 – 402 .
  • Soffer , L. 1992 . “Iodine chemical form in LWR reactor accidents: Regulatory perspective in the United States” . In Proc. The Third CSNI Workshop on Iodine Chemistry in Reactor Safety , Tokai-mura, Japan, Sep. 11–13, 1991, NEA/CSNI/R(91)15, JAERI-M92–012 Edited by: Ishigure , K. , Sacki , M. , Soda , K. and Sugimoto , J.

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