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Solvent Extraction and Ion Exchange Volume 23, 2005 - Issue 1
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Original Articles

Development of a Regenerable Strip Reagent for Treatment of Acidic, Radioactive Waste with Cobalt Dicarbollide‐based Solvent Extraction Processes

Jack D. Law Idaho National Engineering and Environmental Laboratory, P.O. Box 1625, Idaho Falls, ID, 83415‐3870
,
R. Scott Herbst Idaho National Engineering and Environmental Laboratory, P.O. Box 1625, Idaho Falls, ID, 83415‐3870
,
Dean R. Peterman Idaho National Engineering and Environmental Laboratory, P.O. Box 1625, Idaho Falls, ID, 83415‐3870
,
Terry A. Todd Idaho National Engineering and Environmental Laboratory, P.O. Box 1625, Idaho Falls, ID, 83415‐3870
,
Valeriy N. Romanovskiy Khlopin Radium Institute, St. Petersburg, Russia
,
Vasily A. Babain Khlopin Radium Institute, St. Petersburg, Russia
&
Igor V. Smirnov Khlopin Radium Institute, St. Petersburg, Russia
 show all
Pages 59-83 | Received 08 Apr 2004, Accepted 14 Sep 2004, Published online: 15 Sep 2010

References

  • Vanura , P. , Rais , J. , Selucky , P. and Kyrs , M. 1979 . Extraction of strontium with dicarbollide in the presence of polyethylene glycol. Collection of Czechoslovak . Chemical Communications , 44 ( 1 ) : 157 – 166 .
  • Rais , J. and Tachimori , S. 1994 . Extraction separation of tervalent americium and lanthanides in the presence of some soft and hard donors and dicarbollide . Sep. Sci. and Technol. , 29 ( 10 ) : 1347 – 1365 .
  • Romanovskiy , V. N. , Smirnov , I. V. , Babain , V. A. , Todd , T. A. , Herbst , R. S. , Law , J. D. and Brewer , K. N. 2001 . The Universal Solvent Extraction process. I. Development of the UNEX process solvent for the separation of cesium, strontium, and the actinides from acidic radioactive waste . Solvent Extr. Ion Exch. , 19 ( 1 ) : 1 – 21 .
  • Law , J. D. , Herbst , R. S. , Todd , T. A. , Romanovskiy , V. N. , Babain , V. A. , Esimantovskiy , V. M. , Smirnov , I. V. and Zaitsev , B. N. 2001 . The Universal Solvent Extraction (UNEX) process. II. Flowsheet development and demonstration of the UNEX process for the separation of cesium, strontium, and actinides from actual acidic radioactive waste . Solvent Extr. Ion Exch. , 19 ( 1 ) : 23 – 36 .
  • Herbst , R. S. , Law , J. D. , Todd , T. A. , Romanovskiy , V. N. , Babain , V. A. , Esimantovskiy , V. M. , Smirnov , I. V. and Zaitsev , B. N. 2002 . Universal Solvent Extraction (UNEX) flowsheet testing for the removal of cesium, strontium, and actinide elements from radioactive, acidic dissolved calcine waste . Solvent Extr. Ion Exch. , 20 ( 4–5 ) : 429 – 445 .
  • Romanovskiy , V. N. , Babain , V. A. , Smirnov , I. V. , Todd , T. A. , Herbst , R. S. and Law , J. D. 2003 . Regenerable stripping reagents for HLW reprocessing . Proceedings of GLOBAL'03 . November 16–22 2003 , New Orleans, LA. pp. 2239 – 2242 .
  • Wen , N. and Brooker , M. H. 1995 . Ammonium carbonate, ammonium bicarbonate, and ammonium carbamate equilibria: a Raman study . J. Phys. Chem. , 99 : 359 – 368 .
  • Herbst , R. S. , Law , J. D. , Todd , T. A. , Romanovskiy , V. N. , Smirnov , I. V. , Babain , V. A. , Esimantovskiy , V. M. and Zaitsev , B. N. 2003 . Development of the Universal Extraction (UNEX) process for the simultaneous recovery of Cs, Sr, and actinides from acidic radioactive wastes . Sep. Sci. and Technol. , 38 ( 12–13 ) : 2685 – 2708 .
  • Law , J. D. , Herbst , R. S. , Todd , T. A. , Peterman , D. R. , Romanovskiy , V. N. , Esimantovskiy , V. M. , Smirnov , I. V. , Babain , V. A. and Zaitsev , B. N. 2001 . Flowsheet testing of the Universal Extraction Solvent Process for the simultaneous recovery of cesium, strontium, and the actinides from dissolved INEEL calcine . Proceedings Of Waste Management, 2001 . 25 February–1 March 2001 , Tucson, AZ.

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