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Solvent Extraction and Ion Exchange Volume 37, 2019 - Issue 5
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Original Articles

Development of a Selective Americium Separation Process Using H4TPAEN as Water-Soluble Stripping Agent

Cécile MarieCEA, DEN, Research Department on Mining and Fuel Recycling Processes (DMRC), SPDS, LCPE, Bagnols-sur-Cèze cedex, FranceCorrespondence[email protected]
ORCID Iconhttps://orcid.org/0000-0002-4373-0228View further author information
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Peter KaufholzForschungszentrum Jülich GmbH, Institut für Energie- und Klimaforschung - Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyView further author information
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Vincent VanelCEA, DEN, Research Department on Mining and Fuel Recycling Processes (DMRC), SPDS, LCPE, Bagnols-sur-Cèze cedex, FranceORCID Iconhttps://orcid.org/0000-0001-8849-2174View further author information
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Marie-Thérèse DuchesneCEA, DEN, Research Department on Mining and Fuel Recycling Processes (DMRC), SPDS, LCPE, Bagnols-sur-Cèze cedex, FranceView further author information
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Emilie RusselloCEA, DEN, Research Department on Mining and Fuel Recycling Processes (DMRC), SPDS, LCPE, Bagnols-sur-Cèze cedex, FranceView further author information
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Federica FaroldiDipartimento di Scienze Chimiche, della Vita e della Sostenibilità Ambientale, Università degli Studi di Parma, Parma, ItalyORCID Iconhttps://orcid.org/0000-0002-9215-1927View further author information
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Laura BaldiniDipartimento di Scienze Chimiche, della Vita e della Sostenibilità Ambientale, Università degli Studi di Parma, Parma, ItalyORCID Iconhttps://orcid.org/0000-0002-0985-4331View further author information
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Alessandro CasnatiDipartimento di Scienze Chimiche, della Vita e della Sostenibilità Ambientale, Università degli Studi di Parma, Parma, ItalyORCID Iconhttps://orcid.org/0000-0001-9993-3262View further author information
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Andreas WildenForschungszentrum Jülich GmbH, Institut für Energie- und Klimaforschung - Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyORCID Iconhttps://orcid.org/0000-0001-5681-3009View further author information
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Giuseppe ModoloForschungszentrum Jülich GmbH, Institut für Energie- und Klimaforschung - Nukleare Entsorgung und Reaktorsicherheit (IEK-6), Jülich, GermanyORCID Iconhttps://orcid.org/0000-0001-6490-5595View further author information
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Manuel MiguirditchianCEA, DEN, Research Department on Mining and Fuel Recycling Processes (DMRC), SPDS, LCPE, Bagnols-sur-Cèze cedex, FranceORCID Iconhttps://orcid.org/0000-0002-7676-757XView further author information
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Pages 313-327 | Published online: 26 Jul 2019

Citations (20)

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Yufei Wang, Katherine M. Shield & Rebecca J. Abergel. (2023) Hydrophilic Chelators for Aqueous Reprocessing of Spent Nuclear Fuel. Separation & Purification Reviews 0:0, pages 1-19.
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Petr Matveev, Prasanta K. Mohapatra, Stepan N. Kalmykov & Vladimir Petrov. (2021) Solvent extraction systems for mutual separation of Am(III) and Cm(III) from nitric acid solutions. A review of recent state-of-the-art. Solvent Extraction and Ion Exchange 39:7, pages 679-713.
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Andreas Geist & Petra J. Panak. (2021) Recent Progress in Trivalent Actinide and Lanthanide Solvent Extraction and Coordination Chemistry with Triazinylpyridine N Donor Ligands. Solvent Extraction and Ion Exchange 39:2, pages 128-151.
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Manuel Miguirditchian, Vincent Vanel, Cécile Marie, Vincent Pacary, Marie-Christine Charbonnel, Laurence Berthon, Xavier Hérès, Marc Montuir, Christian Sorel, Marie-Jordane Bollesteros, Sylvain Costenoble, Christine Rostaing, Michel Masson & Christophe Poinssot. (2020) Americium Recovery from Highly Active PUREX Raffinate by Solvent Extraction: The EXAm Process. A Review of 10 Years of R&D. Solvent Extraction and Ion Exchange 38:4, pages 365-387.
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Articles from other publishers (16)

Iván Sánchez-García, Richard J.M. Egberink, Willem Verboom & Hitos Galán. (2024) Gamma radiolysis studies of N,N-dioctyl-2-hydroxyacetamide: Complexation effect on the stability and implications on the hydrometallurgical extraction performance. Radiation Physics and Chemistry 214, pages 111299.
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Iván Sánchez-García & Hitos Galán. (2023) Effect of Europium Complexation on N,N,N′,N′-Tetraoctyldiglycolamide Degradation Against Gamma Radiation. Arabian Journal for Science and Engineering.
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P. Zsabka, A. Wilden, K. Van Hecke, G. Modolo, M. Verwerft & T. Cardinaels. (2023) Beyond U/Pu separation: Separation of americium from the highly active PUREX raffinate. Journal of Nuclear Materials 581, pages 154445.
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Gregory P. Horne, Cristian Celis-Barros, Jacy K. Conrad, Travis S. Grimes, Jeffrey R. McLachlan, Brian M. Rotermund, Andrew R. Cook & Stephen P. Mezyk. (2023) Impact of lanthanide ion complexation and temperature on the chemical reactivity of N , N , N ′, N ′-tetraoctyl diglycolamide (TODGA) with the dodecane radical cation . Physical Chemistry Chemical Physics 25:24, pages 16404-16413.
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Hang Zhang, Yin-Yong Ao, Yue Wang, Shang-Jie Zhao, Jia-Yang Sun, Mao-Lin Zhai, Jiu-Qiang Li, Jing Peng & Hui-Bo Li. (2023) Effect of radiolysis of TODGA on the extraction of TODGA/n-dodecane toward Eu(III): an experimental and DFT study. Nuclear Science and Techniques 34:4.
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Andreas Wilden, Dimitri Schneider, Zaina Paparigas, Maximilian Henkes, Fabian Kreft, Andreas Geist, Eros Mossini, Elena Macerata, Mario Mariani, Maria Chiara Gullo, Alessandro Casnati & Giuseppe Modolo. (2022) Selective actinide(III) separation using 2,6-bis[1-(propan-1-ol)-1,2,3-triazol-4-yl]pyridine (PyTri-Diol) in the innovative-SANEX process: laboratory scale counter current centrifugal contactor demonstration. Radiochimica Acta 110:6-9, pages 515-525.
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Joseph A. Mattocks, Joseph A. Cotruvo & Gauthier J.-P. Deblonde. (2022) Engineering lanmodulin's selectivity for actinides over lanthanides by controlling solvent coordination and second-sphere interactions. Chemical Science 13:20, pages 6054-6066.
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Ashleigh Kimberlin, Georges Saint-Louis, Dominique Guillaumont, Béatrice Camès, Philippe Guilbaud & Laurence Berthon. (2022) Effect of metal complexation on diglycolamide radiolysis: a comparison between ex situ gamma and in situ alpha irradiation . Physical Chemistry Chemical Physics 24:16, pages 9213-9228.
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Helena Singer, Björn Drobot, Cathleen Zeymer, Robin Steudtner & Lena J. Daumann. (2021) Americium preferred: lanmodulin, a natural lanthanide-binding protein favors an actinide over lanthanides. Chemical Science 12:47, pages 15581-15587.
Crossref
Amit Pandey, S. Hashmi, G. Salunkhe, Velavan Kathirvelu, Keisham S. Singh, Rohit Singh Chauhan & Arijit Sengupta. (2021) Tuning the extraction mechanism of uranyl ion in bicyclooctanium, propylpyridinium, piperidinium and imidazolium based ionic liquids: First ever evidence of 'cation exchange', 'anion exchange' and 'solvation' mechanism. Journal of Molecular Liquids 337, pages 116435.
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T. Kooyman. (2021) Current state of partitioning and transmutation studies for advanced nuclear fuel cycles. Annals of Nuclear Energy 157, pages 108239.
Crossref
Jinlong Fan, Li Duan, Yufeng Wang & Ping Huang. (2021) Assembly of a polymer-based extraction resin and separation of minor actinides. Colloids and Surfaces A: Physicochemical and Engineering Aspects 610, pages 125473.
Crossref
Peter R. Zalupski, Travis S. Grimes, Corey D. Pilgrim, Colt R. Heathman, Santa Jansone-Popova, Katherine R. Johnson, Vyacheslav Bryantsev & Robert C. ChapleskiJrJr. 2021. Including Actinides. Including Actinides 1 162 .
Andreas Wilden, Fabian Kreft, Dimitri Schneider, Zaina Paparigas, Giuseppe Modolo, Gregg J. Lumetta, Artem V. Gelis, Jack D. Law & Andreas Geist. (2020) Countercurrent Actinide Lanthanide Separation Process (ALSEP) Demonstration Test with a Simulated PUREX Raffinate in Centrifugal Contactors on the Laboratory Scale. Applied Sciences 10:20, pages 7217.
Crossref
O. V. Kharitonov, L. A. Firsova & E. A. Kozlitin. (2020) All-chromatographic method for the recovery of Americium-241 from solutions of complex composition. Journal of Radioanalytical and Nuclear Chemistry 326:1, pages 627-636.
Crossref
Patrik Weßling, Udo Müllich, Elise Guerinoni, Andreas Geist & Petra J. Panak. (2020) Solvent extraction of An(III) and Ln(III) using TODGA in aromatic diluents to suppress third phase formation. Hydrometallurgy 192, pages 105248.
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