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Original Article

Investigation of Absorption and Scattering Properties of Soot Aggregates of Different Fractal Dimension at 532 nm Using RDG and GMM

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Pages 1393-1405 | Received 01 Jun 2013, Accepted 09 Sep 2013, Published online: 10 Oct 2013

Figures & data

Table 1 Four different expressions for the structure factor considered in this study

Figure 1 Typical fractal aggregates generated using the tunable cluster–cluster aggregation algorithm, except the smallest aggregates shown for Np = 20. These aggregates are of size Np = 20, 50, 100, 200, and 400, respectively, for (a) Df = 1.4, (b) Df = 1.78, and (c) Df = 2.1. In all cases, kf = 2.3 and dp = 30 nm.
Figure 1 Typical fractal aggregates generated using the tunable cluster–cluster aggregation algorithm, except the smallest aggregates shown for Np = 20. These aggregates are of size Np = 20, 50, 100, 200, and 400, respectively, for (a) Df = 1.4, (b) Df = 1.78, and (c) Df = 2.1. In all cases, kf = 2.3 and dp = 30 nm.
Figure 2 Comparison of RDG nondimensional vertical–vertical differential scattering cross-sections with four different structure factors for monodisperse aggregates of Np = 50 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases, λ = 532 nm, dp = 30 nm, and kf = 2.3. The corresponding GMM results are also plotted. (Color figure available online.)
Figure 2 Comparison of RDG nondimensional vertical–vertical differential scattering cross-sections with four different structure factors for monodisperse aggregates of Np = 50 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases, λ = 532 nm, dp = 30 nm, and kf = 2.3. The corresponding GMM results are also plotted. (Color figure available online.)
Figure 3 Comparison of RDG nondimensional vertical–vertical differential scattering cross-sections with four different structure factors for monodisperse aggregates of Np = 200 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases, λ = 532 nm, dp = 30 nm, and kf = 2.3. The corresponding GMM results are also plotted. (Color figure available online.)
Figure 3 Comparison of RDG nondimensional vertical–vertical differential scattering cross-sections with four different structure factors for monodisperse aggregates of Np = 200 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases, λ = 532 nm, dp = 30 nm, and kf = 2.3. The corresponding GMM results are also plotted. (Color figure available online.)
Figure 4 Comparison of nondimensional vertical–vertical differential scattering cross-sections predicted by RDG and GMM for ensembles of monodisperse aggregate of Np = 800 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases: λ = 532 nm, dp = 30 nm, and kf = 2.3. (Color figure available online.)
Figure 4 Comparison of nondimensional vertical–vertical differential scattering cross-sections predicted by RDG and GMM for ensembles of monodisperse aggregate of Np = 800 and different fractal dimensions: (a) against qRg, (b) against the scattering angle θ. In all cases: λ = 532 nm, dp = 30 nm, and kf = 2.3. (Color figure available online.)
Figure 5 Variation of the nondimensional total scattering cross-section with aggregate size for aggregates of different fractal dimensions: (a) Df = 2.1, (b) Df = 1.78, and (c) Df = 1.4. (Color figure available online.)
Figure 5 Variation of the nondimensional total scattering cross-section with aggregate size for aggregates of different fractal dimensions: (a) Df = 2.1, (b) Df = 1.78, and (c) Df = 1.4. (Color figure available online.)
Figure 6 Variation of the asymmetry factor with aggregate size for monodisperse aggregates of different fractal dimension. (Color figure available online.)
Figure 6 Variation of the asymmetry factor with aggregate size for monodisperse aggregates of different fractal dimension. (Color figure available online.)
Figure 7 Variation of nondimensional aggregate absorption cross-section with aggregate size for monodisperse aggregates of different fractal dimension. (Color figure available online.)
Figure 7 Variation of nondimensional aggregate absorption cross-section with aggregate size for monodisperse aggregates of different fractal dimension. (Color figure available online.)
Supplemental material

SupplementaryInfo_Liu_etal.zip

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