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Molecular Physics
An International Journal at the Interface Between Chemistry and Physics
Volume 51, 1984 - Issue 1
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Original Articles

Raman spectra of fluid N2

Temperature and density behaviour of the second momentFootnote

Work supported by GNSM (CNR) and MPI.

&
Pages 97-117 | Received 09 Jun 1983, Accepted 17 Jul 1983, Published online: 22 Aug 2006

References

  • See references mentioned in [2 (a)] for data before 1973 Dardy H.D. Volterra V. Litovitz T.A. J. chem. Phys. 1973 59 4491 4491 Shoen, P. E., Cheung, P. S. Y., Jackson, D. A., and Powles, J. G., 1975, Molec. Phys., 29, 1197. Bruining, J., and Clarke, J. H. R., 1976, Molec. Phys., 31, 1425. Van Konynenburg, P., and Steele, W. A., 1975, J. chem. Phys., 62, 2301. Gill, E. B., and Steele, D., 1977, Molec. Phys., 34, 231. Langer, H., and Versmold, H., 1979, Ber. Bunsenges. phys. Chem., 83, 510. Versmold, H., 1981, Molec. Phys., 43, 383. Perrot, M., Bouachir, M., and Lascombe, J., 1981, Molec. Phys., 42, 551. Andreani, C., Morales, P., and Rocca, D., 1981, Molec. Phys., 44, 445.
  • Laulicht , I. and Meirman , S. 1973 . J. chem. Phys. , 59 : 2521 – 2521 . (b) Wright, R. B., Schwartz, M., and Wang, C. H., 1973, J. chem. Phys., 58, 5125. (c) Schroeder, J., Schiemann, V. H., and Jonas, J., 1978, J. chem. Phys., 69, 5479.
  • Frenkel , D. and McTague , J.P. 1980 . J. chem. Phys. , 72 : 2801 – 2801 .
  • Hanson , F.E. and McTague , J.P. 1980 . J. chem. Phys. , 72 : 1733 – 1733 .
  • De Santis , A. , Moretti , E. and Sampoli , M. 1982 . Molec. Phys. , 46 : 1271 – 1271 .
  • De Santis , A. and Sampoli , M. Phenomena Induced by Intermolecular Interactions , Proc. NATO Adv. Res. Workshop . (in the press)
  • Ladanyi , B.M. 1983 . J. chem. Phys. , 78 : 2189 – 2189 .
  • Gordon , R.G. 1964 . J. chem. Phys. , 40 : 1973 – 1973 . St. Pierre, A. G., and Steele, W. A., 1981, Molec. Phys., 43, 123.
  • Bansal , M.L. , Deb , S.K. and Roy , A.P. 1981 . Chem. Phys. Lett. , 83 : 83 – 83 .
  • Keyes , T. , Kivelson , D. and McTague , J.P. 1971 . J. chem. Phys. , 55 : 4096 – 4096 .
  • Ladanyi , B.M. and Keyes , T. 1977 . Molec. Phys. , 33 : 1063 – 1063 .
  • Keyes , T. and Ladanyi , B.M. 1977 . Molec. Phys. , 33 : 1099 – 1099 .
  • Battaglia , M.R. , Cox , T.I. and Madden , P.A. 1979 . Molec. Phys. , 37 : 1413 – 1413 .
  • See and references quoted therein Frenkel D. McTague J.P. J. chem. Phys. 1980 72 2801 2801
  • Kielich , S. 1982 . J. Phys. , 43 : 1749 – 1749 . and references quoted therein.
  • Madden , P.A. 1978 . Molec. Phys. , 36 : 365 – 365 . Guillot, B., Bratos, S., and Birnbaum, G., 1980, Phys. Rev. A, 22, 2230. Madden, P. A., and Cox, T. I., 1981, Molec. Phys., 43, 287.
  • Balucani , U. and Vallauri , R. 1979 . Molec. Phys. , 38 : 1099 – 1099 . 1979, Ibid., 38, 1115.
  • Shelton , D.P. , Tabisz , G.C. , Barocchi , F. and Zoppi , M. 1982 . Molec. Phys. , 46 : 21 – 21 .
  • Barocchi , F. , Moraldi , M. and Zoppi , M. 1982 . Phys. Rev. A , 26 : 2168 – 2168 . Barocchi, F. Zoppi, M., and Neumann, M., 1983, Phys. Rev. A, 27, 1587.
  • Cox , T.I. , Battaglia , M.R. and Madden , P.A. 1979 . Molec. Phys. , 38 : 1539 – 1539 .
  • Cox , T.I. and Madden , P.A. 1980 . Molec. Phys. , 39 : 1487 – 1487 .
  • Berrue , T. , Chave , A. , Dumon , B. and Thibeau , M. 1978 . J. Phys. , 39 : 815 – 815 .
  • Rose , M.E. 1957 . Elementary Theory of Angular Momentum , John Wiley & Sons . Edmonds, A. R., 1957, Angular Momentum in Quantum Mechanics (Princeton University Press).
  • Frenkel , D. 1980 . Proc. Int. School of Physics ‘Enrico Fermi’ , Edited by: Van Kranendonk , J. Vol. LXXV , Bologna . Stone, A. J., 1975, Molec. Phys., 29, 1461.
  • Bratos , S. and Marechal , E. 1971 . Phys. Rev. A , 4 : 1078 – 1078 . Clouter, M. J., Kiefte, H., and Jain, R. K., 1980, J. chem. Phys., 73, 673.
  • Pecora , R. and Steele , W.A. 1966 . J. chem. Phys. , 42 : 1872 – 1872 .
  • See Gordon R.G. J. chem. Phys. 1964 41 1819 1819 recall that the second moment of Raman bands is equal to three times that for I.R. absorption bands.
  • Hansen , J.P. and McDonald , I.R. 1976 . Theory of Simple Liquids , Academic Press .
  • From our findings it results that if we put α′ = α and γ′ = γ the contribution of S 2 in RAM is twice than in RAY whereas that of S 3 is the same in both. The RAY result agrees with the Kielich one Kielich S. J. Phys. 1982 43 1749 1749 [15] derived using the formalism of irreducible cartesian tensors.
  • De Santis , A. , Nardone , M. , Sampoli , M. , Morales , P. and Signorelli , G. 1980 . Molec. Phys. , 39 : 913 – 913 .
  • De Santis , A. , Nardone , M. and Sampoli , M. 1980 . Molec. Phys. , 41 : 769 – 769 . (b) Sampoli, M., De Santis, A., and Nardone, M., 1981, Can. J. Phys., 59, 1403.
  • Jacobsen , R.T. , Stewart , R.B. , McCarty , R.D. and Hanley , H.J.M. 1973 . Natn. Bur. Stand. Tech. Note , : 648 – 648 .
  • Weber , W.A. 1979 . Spectroscopy of gases and liquids , Edited by: Weber , A. Springer-Verlag .
  • Alder , B.J. , Strauss , H.L. and Weis , J.J. 1975 . J. chem. Phys. , 62 : 2328 – 2328 .
  • Courtois , D. and Jouve , P. 1975 . J. molec. Spectrosc. , 55 : 18 – 18 . Bridge, N. J., and Buckingham, A. D., 1966, Proc. R. Soc. A, 295, 334.
  • In equations (5) of reference De Santis A. Moretti E. Sampoli M. Molec. Phys. 1982 46 1271 1271 [5] there are obvious errors. It should read Ω ij (l) instead of Ω ij (l) and instead of in equations (5 b) and (5 c) respectively.
  • Ladd , A.J.C. , Litovitz , T.A. and Montrose , C.J. 1979 . J. chem. Phys. , 71 : 4242 – 4242 . Alder, B. J., Weis, J. J., and Strauss, H. L., 1973, Phys. Rev. A, 7, 281.
  • The adopted value of 0.1 has to be regarded as a very rough estimate Indeed all fluid N2 simulations [3, 39] give g 2 with large statistical errors; moreover g 2 has been found to depend significantly on size and shape of the cutting volume [40].
  • Levesque , D. and Weis , J.J. 1975 . Phys. Rev. A , 12 : 2538 – 2538 .
  • Impey , R.W. , Madden , P.A. and Tildesley , D.J. 1981 . Molec. Phys. , 44 : 1319 – 1319 .
  • Breuer , G. 1982 . Molec. Phys. , 45 : 349 – 349 .
  • Singer , K. , Taylor , A. and Singer , J.V.L. 1977 . Molec. Phys. , 33 : 1757 – 1757 .

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