Preparation, Characterization, and Properties of Novel Polyimide–SiO₂ Hybrid Composites Based on Bipyridine for Low Dielectric Applications

REFERENCES

• Lee, H.S.; Lee, A.S.; Baek, K.Y.; Hwang, S.S. Low dielectric materials for microelectronics. In: Silaghi, M.A. ed. Dielectric Material, InTech: Rijeka, Croatia, 2012, Chapter 3; pp. 60–76.
   Google Scholar
• Ho, P.S.; Leu, J.; Lee, W.W. Low Dielectric Constant Materials for IC Applications, Springer-Verlag Heidelberg, Berlin, 2003, pp. 1–4.
   Google Scholar
• Seçkin, T.; Köytepe, S.; Adıgüzel, H.I. Molecular design of POSS core star polyimides as a route to low-κ dielectric materials. Mater. Chem. Phys. 2008, 112, 1040–1046.
   Web of Science ®Google Scholar
• Zhang, C.; Xu, H.Y.; Zhao, X. Structure and properties of low-dielectric-constant poly(acetoxystyrene-co-octavinyl-polyhedral oligomeric silsesquioxane) hybrid nanocomposite. Chin. Chem. Lett. 2010, 21, 488–491.
   Web of Science ®Google Scholar
• Sun, J.; Zhang, Q.; Gu, J.; Zhang, J.; Ai, Q. Preparation and characterization of polyimide-silica hybrid thin films. Polym. Plast. Technol. Eng. 2010, 49 (3), 250–253.
   Web of Science ®Google Scholar
• Mallakpour, S.; Abdolmaleki, A.; Rostami, M. Morphological and thermal properties of poly(amide-imide)/ZnO nanocomposites derived from 4,4′-methylenebis(3-chloro-2,6-diethyl trimellitimidobenzene) and 3,5-diamino-N-(4-hydroxyphenyl)benzamide. Polym. Plast. Technol. Eng. 2014, 53 (15), 1615–1624.
   Web of Science ®Google Scholar
• Fu, H.K.; Kuo, S.W.; Yeh, D.R.; Chang, F.C. Properties enhancement of PS nanocomposites through the POSS surfactants. J. Nanomater. 2008, Article ID 739613, 2008. 1–7. doi:10.1155/2008/739613
   Web of Science ®Google Scholar
• Vural, S.; Köytepe, S.; Seçkin, T.; Adıgüzel, I. Synthesis, characterization and dielectric properties of rodlike zinc oxide-polyimide nanocomposites. Polym. Plast. Technol. Eng. 2012, 51 (4), 369–376.
   Web of Science ®Google Scholar
• Pan, B.; Cheng, Y.; Wang, Y.; Feng, Y.; Ye, W.; Tian, Y.; Wang, X. Polydicyclopentadiene reinforced with grafted silica nanoparticles. Polym. Plast. Technol. Eng. 2013, 52 (6), 586–591.
   Web of Science ®Google Scholar
• Chang, C.-C.; Chen, W.-C. Synthesis and optical properties of polyimide-silica hybrid thin films. Chem. Mater. 2002, 14, 4242–4248.
   Web of Science ®Google Scholar
• Ye, X.; Wang, J.; Xu, Y.; Niu, L.; Fan, Z.; Gong, P.; Ma, L.; Wang, H.; Yang, Z.; Yang, S. Mechanical properties and thermostability of polyimide/mesoporous silica nanocomposite via effectively using the pores. J. Appl. Polym. Sci. 2014, 131 (23), 41173–41180.
   Web of Science ®Google Scholar
• Martin, S.J.; Godschalx, J.P.; Mills, M.E.; Shaffer, E.O.; Townsend, P.H. Development of a low-dielectric-constant polymer for the fabrication of integrated circuit interconnect. Adv. Mater. 2000, 12, 1769–1778.
   Web of Science ®Google Scholar
• Kreuz, J.A.; Edman, J.R. Polyimide films. Adv. Mater. 1998, 10, 1229–1232.
   Web of Science ®Google Scholar
• Vora, R.H.; Krishnan, P.S.G.; Goh, S.H.; Chung, T.-S. Synthesis and properties of designed low-k fluoro-copolyetherimides. Adv. Funct. Mater. 2001, 11, 361–373.
   Web of Science ®Google Scholar
• Enhessari, M.; Shaterian, M.; Ozaee, K.; Karamali, E. Synthesis and thermal properties of polyimide/BaZrO3 novel nanocomposites. Polym. Plast. Technol. Eng. 2012, 51 (4), 345–349.
   Web of Science ®Google Scholar
• Li, J. Effect of silane coupling agent on the tensile properties of carbon fiber-reinforced thermoplastic polyimide composites. Polym. Plast. Technol. Eng. 2010, 49 (4), 337–340.
   Web of Science ®Google Scholar
• Gunasekaran, S.G.; Dharmendirakumar, M. Siloxane core-modified organo soluble novel polyimide/multi-walled carbon nanotube nanocomposites. Polym. Plast. Technol. Eng. 2014, 53 (9), 903–916.
   Web of Science ®Google Scholar
• Tiwari, A.; Gupta, M.K.; Pandey, K.N.; Mathur, G.N.; Nema, S.K. Encapsulation of air-filled poly(dimethylsiloxane) microballoons in polyimide as a polymeric low ε dielectric. Polym. Int. 2004, 53, 1744–1751.
   Web of Science ®Google Scholar
• Jain, S.; Goossens, H.; Picchioni, F.; Magusin, P.; Mezari, B.; Duin, M.V. Synthetic aspects and characterization of polypropylene–silica nanocomposites prepared via solid-state modification and sol–gel reactions. Polymer 2005, 46, 6666–6681.
   Web of Science ®Google Scholar
• Fasce, D.P.; dell’Erba, I.E.; Williams, R.J.J. Synthesis of a soluble functionalized-silica by the hydrolysis and condensation of organotrialkoxysilanes bearing (β-hydroxy) tertiary amine groups with tetraethoxysilane. Polymer 2005, 46, 6649–6656.
   Web of Science ®Google Scholar
• Tommalieh, M.J.; Zihlif, A.M.; Ragosta, G. Electrical and thermal properties of polyimide/silica nanocomposite. J. Exp. Nanosci. 2011, 6 (6), 652–664.
   Web of Science ®Google Scholar
• Musto, P.; Ragosta, G.; Scarinzi, G.; Mascia, L. Polyimide-silica nanocomposites: Spectroscopic, morphological and mechanical investigations. Polymer 2004, 45, 1697–1706.
   Web of Science ®Google Scholar
• Chen, B.-K.; Chiu, T.-M.; Tsay, S.-Y. Synthesis and characterization of polyimide/silica hybrid nanocomposites. J. Appl. Polym. Sci. 2004, 94, 382–393.
   Web of Science ®Google Scholar
• Musto, P.; Ragosta, G.; Scarinzi, G.; Mascia, L. Toughness enhancement of polyimides by in situ generation of silica particles. Polymer 2004, 45, 4265–4274.
   Web of Science ®Google Scholar
• Zou, H.; Wu, S.; Shen, J. Polymer/Silica nanocomposites: Preparation, characterization, properties, and applications. Chem. Rev. 2008, 108 (9), 3893–3957.
   PubMed Web of Science ®Google Scholar
• Shantalii, T.A.; Karpova, I.L.; Dragan, K.S.; Privalko, E.G.; Privalko, V.P. Synthesis and thermomechanical characterization of polyimides reinforced with the sol–gel derived nanoparticles. Sci. Technol. Adv. Mater. 2003, 4, 115–119.
   Web of Science ®Google Scholar
• Wu, C.-S. Synthesis of polyethylene-octene elastomer/SiO2-TiO2 nanocomposites via in situ polymerization: Properties and characterization of the hybrid. J. Polym. Sci., Part A: Polym. Chem. 2005, 43, 1690–1701.
   Web of Science ®Google Scholar
• Yu, Y.-Y.; Chein, W.-C.; Tsai, T.-W. High transparent soluble polyimide/silica hybrid optical thin films. Polym. Test. 2010, 29, 33–40.
   Web of Science ®Google Scholar
• Kim, Y.-J.; Kim, J.-H.; Ha, S.-W.; Kwon, D.; Lee, J.-K. Polyimide nanocomposites with functionalized SiO2 nanoparticles: Enhanced processability, thermal and mechanical properties. RSC Adv. 2014, 4 (82), 43371–43377.
   Google Scholar
• Bershtein, V.A.; Egorova, L.M.; Yakushev, P.N.; Pissis, P.; Sysel, P.; Brozova, L. Molecular dynamics in nanostructured polyimide–silica hybrid materials and their thermal stability. J. Polym. Sci. Part B: Polym. Phys. 2002, 40, 1056–1069.
   Web of Science ®Google Scholar
• Ismail, H.; Ahmad, H.S. The Properties of acrylonitrile-butadiene rubber (NBR) composite with halloysite nanotubes (HNTs) and silica or carbon black. Polym. Plast. Technol. Eng. 2013, 52 (12), 1175–1182.
   Web of Science ®Google Scholar
• Tsai, M.-H.; Whang, W.-T. Low dielectric polyimide/poly(silsesquioxane)-like nanocomposite material. Polymer 2001, 42, 4197–4207.
   Web of Science ®Google Scholar
• Kıvılcım, N.; Seçkin, T.; Köytepe, S. Porous pyridine based polyimide–silica nanocomposites with low dielectric constant. J. Porous Mater. 2013, 20 (4), 709–718.
   Web of Science ®Google Scholar
• Kramarenko, V.Y.; Shantalii, T.A.; Karpova, I.L.; Dragan, K.S.; Privalko, E.G.; Privalko, V.P.; Fragiadakis, D.; Pissis, P. Polyimides reinforced with the sol–gel derived organosilicon nanophase as low dielectric permittivity materials. Polym. Adv. Technol. 2004, 15, 144–148.
   Web of Science ®Google Scholar
• Zhao, G.; Ishizaka, T.; Kasai, H.; Hasegawa, M.; Furukawa, T.; Nakanishi, H.; Oikawa, H. Ultralow-dielectric-constant films prepared from hollow polyimide nanoparticles possessing controllable core sizes. Chem. Mater. 2009, 21 (2), 419–424.
   Web of Science ®Google Scholar