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Technical Paper

Mobility and Criticality of Plutonium in a Repository

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Pages 309-321 | Published online: 10 Apr 2017

References

  • “Vereinbarung zwischen der Bundesregierung und den Energieversorgungs-unternehmen vol 14, Juni 2000, Anlage
  • “Erklärung des Bundes zur Erkundung des Salzstockes in Gorleben”; available on the Internet at 〈http://www.bmu.de/fset1024.php〉 (2000).
  • W. E. KASTENBERG, P. F. PETERSON, J. AHN, J. BURCH, G. CASHER, P. L. CHAMBRé, E. GREENSPAN, D. R. OLANDER, and J. L. VUJIC, “Considerations of Autocatalytic Criticality of Fissile Materials in Geologic Repositories,” Nucl. Technol., 115, 298 (1996).
  • E. GREENSPAN, J. VUJIC, and J. BURCH, “Neutronic Analysis of Critical Configurations in Geologic Repositories: I—Weapons-Grade Plutonium,” Nucl. Sci. Eng., 127, 262 (1997).
  • J. VUJIC and E. GREENSPAN, “Neutronic Analysis of Critical Configurations in Geologic Repositories: II—Highly Enriched Uranium,” Nucl. Sci. Eng., 129, 1 (1998).
  • K.-D. CLOSS, Anforderung an Plutonium-Abfallprodukte aus der Sicht der Endlagerung, W. BLUM, Ed.; “Energie Plutonium-Strom und die Umwelt: 17 Vorträge der Tagungen Heidelberg (1999) und Dresden (2000),” Deutsche Physikalische Gesellschaft (DPG), 69 (2000); available on the Internet at 〈http://www.dpgphysik.de/fachgremien/ake/tagungsband9900.pdf〉.
  • R. NAUDET, “The Oklo Nuclear Reactors: 1800 Million Years Ago,” Interdiscip. Sci. Rev., 1, 1, 72 (1976).
  • C.H.R. KüPPERS, W. LIEBERT, and M. SAILER, “Alternative Wege zur Behandlung von Plutonium,” Proc. Workshop Optionen bei der Verwertung und Entsorgung von Plutonium, Jülich, Germany, January 13–14, 2000.
  • P. BRENNECKE and E. WARNECKE, “Provisional Konrad Disposal Conditions, Table 7,” in “Betonbehälter Typ I,” ET-3/90, Bundesamt für Strahlenschutz, Salzgitter (1990).
  • H. SPILKER, “Status of the Development of Disposal Casks and Prospects in Germany,” Proc. Dis Tec’98, Hamburg, Germany, September 9–11, 1998, p. 301, Kontec, Hamburg (1998).
  • A. PUDEWILLS, N. MüLLER-HOEPPE, and R. PAPP, “Thermal and Thermomechanical Analyses for Disposal in Drifts of a Repository in Rock Salt,” Nucl. Technol., 112, 79 (1995).
  • W. BECHTHOLD, T. ROTHFUCHS, A. POLEY, M. GHOREYCHI, S. HEUSERMANN, A. GENS, and S. OLIVELLA, “Backfilling and Sealing of Underground Repositories for Radioactive Waste in Salt (BAMBUS Project),” EUR-19124-EN, European Commission (1999).
  • B. KIENZLER, B. LUCKSCHEITER, and S. WILHELM, “Waste from Corrosion Modeling: Comparison with Experimental Results,” Waste Manage., 21, 8, 741 (2001).
  • M. KELM and E. BOHNERT, “Radiation Chemical Effects in the Near Field of a Final Disposal Site—I: Radiolytic Products Formed in Concentrated NaCl Solutions,” Nucl. Technol., 129, 119 (2000).
  • R. J. SILVA and H. NITSCHE, “Actinide Environmental Chemistry,” Radiochim. Acta, 70/71, 377 (1995).
  • K. SPAHIU, L. WERME, and U.-B. EKLUND, “The Influence of Near-Field Hydrogen on Actinide Solubilities and Spent Fuel Leaching,” Radiochim. Acta, 88, 507 (2000).
  • B. GRAMBOW, A. LOIDA, A. MARTINEZ-ESPARZA, P. DIAZ AROCAS, J. DE PABLO, J. L. PAUL, G. MARX, J. P. GLATZ, K. LEMMENS, K. OLLILIA, and H. CHRISTENSEN, “Long-Term Safety of Radioactive Waste Disposal: Source Term for Performance Assessment of Spent Fuel as a Waste Form,” Final Report FZKA 6420, Forschungszentrum Karlsruhe (2000).
  • A. LOIDA, B. GRAMBOW, H. KLEYKAMP, P. DRESSLER, and H. D. GOTTSCHALG, “Langzeitsicherheit der Endlagerung radioaktiver Abfälle: Korrosionsuntersuchungen an hochabgebranntem LWR-UO2 Kernbrennstoff unter dynamischen Bedingungen,” FZKA 5674, Forschungszentrum Karlsruhe (1995).
  • B. GRAMBOW, A. LOIDA, P. DRESSLER, H. GECKEIS, J. GAGO, I. CASAS, J. DE PABLO, J. GIMENEZ, and M. E. TORRERO, “Long-Term Safety of Radioactive Waste Disposal: Chemical Reaction of Fabricated and High Burnup Spent UO2 Fuel with Saline Brines,” final report FZKA 5702, Forschungszentrum Karlsruhe (1996).
  • B. KIENZLER and V. METZ, “Status of Source Term Modeling for Radioactive Wastes in Germany,” Proc. 9th Int. High-Level Radioactive Waste Management Conf., Las Vegas, Nevada, April 29–May 3, 2001, American Nuclear Society (2001) (CD-ROM).
  • V. NECK, T. H. FANGHäNEL, G. RUDOLPH, and J. I. KIM, “Thermodynamics of Neptunium (V) in Concentrated Salt Solutions: Chloride Complexation and Ion Interaction (Pitzer) Parameters for the NpO+2 Ion,” Radiochim. Acta, 69, 39 (1995).
  • V. NECK and J. I. KIM, “Solubility and Hydrolysis of Tetravalent Actinides,” FZKA 6350, Forschungszentrum Karlsruhe (1999).
  • I. GRENTHE, J. FUGER, R. J. M. KONINGS, R. J. LEMIRE, A. B. MULLER, C. NGUYEN-TRUNC, and H. WANNER, Chemical Thermodynamics of Uranium, North-Holland, Amsterdam (1992).
  • P. DIAZ AROCAS and B. GRAMBOW, “Solid-Liquid Phase Equilibria of U (VI) in NaCl Solutions,” Geochim. Cosmochim. Acta, 62, 2, 245 (1998).
  • J. BRUNO, I. GRENTHE, and M. MUÑOZ, “Studies on the Radionuclide Coprecipitation-Solid Solution Formation. The UO2 (s)-La (OH)3 (s) Coprecipitation as an Analogue for the UO2 (s)-Pu (OH)3 (s) System,” Mat. Res. Soc., Symp. Proc., 50, 717 (1985).
  • J. H. VAN’T HOFF, “Über feste Lösungen und Molekulargewichtsbestimmung an festen Körpern,” Z. Physik. Chem., 5, 322 (1890).
  • H. W. B. ROOZEBOOM, “Über die Löslichkeit von Mischkrystallen, speziell zweier isomorpher Körper,” Z. Physik. Chem., 8, 504 (1891).
  • J. INCZéDY, T. LENGYEL, and A. M. URE, Compendium of Analytical Nomenclature. Definitive Rules 1977, 3rd ed., International Union of Pure and Applied Chemistry; available on the Internet at 〈http://www.iupac.org/publications/analytical_compendium/Cha09sec50.pdf〉 (1997).
  • J. QUINONES, B. GRAMBOW, A. LOIDA, and H. GECKEIS, “Coprecipitation Phenomena During Spent Fuel Dissolution. Part 1: Experimental Procedure and Initial Results on Trivalent Ion Behaviour,” J. Nucl. Mater., 238, 38 (1996).
  • B. GRAMBOW, E. SMAILOS, H. GECKEIS, R. MüLLER, and H. HENTSCHEL, “Sorption and Reduction of Uranium (VI) on Iron Corrosion Products Under Reducing Saline Conditions,” Radiochim. Acta, 74, 149 (1996).
  • CRC Handbook of Chemistry and Physics, 77th ed., CRC Press, Boca Raton, Florida (1997).
  • T. T. VANDERGRAAF, K. V. TICKNOR, and T. W. MELNYK, “The Selection of a Sorption Data Base for the Geosphere Model in the Canadian Nuclear Fuel Waste Management Program,” J. Contaminant Hydrol., 13, 327 (1993).
  • B. KIENZLER, P. VEJMELKA, and V. METZ, “Near Field Radionuclide Concentrations: Sorption or Solubility Constrained?” presented at 8th Int. Conf. Radioactive Waste Management and Environmental Remediation (ICEM’01), Brugges, Belgium, September 30–October 4, 2001.
  • B. KIENZLER, J. RöMER, P. VEJMELKA, M. JANSSON, T. E. ERIKSEN, and K. SPAHIU, “Actinide Migration in Granite Fractures: Comparison Between In-Situ and Laboratory Results,” presented at Materials Research Society Conf. Scientific Basis of Nuclear Waste Management XXVI, Boston, Massachusetts, December 2–6, 2002.
  • J. AHN and S. NAKAYAMA, “Modeling for Migration of a Redox-Sensitive Radionuclide in Engineered Barriers,” Nucl. Technol., 97, 323 (1992).
  • C. K. D. HSI and D. LANGMUIR, “Adsorption of Uranyl onto Ferric Oxyhydroxides: Application of the Surface Complexation Site Binding Model,” Geochim. Cosmochim. Acta, 49, 1931 (1985).
  • B. GMAL, E. F. MOSER, and W. WEBER, “Criticality Safety Analysis for the Post-Operational Phase of a Final Repository in Germany,” Proc. Annual Mtg. Nuclear Technology ’99, p. 363, Inforum Bonn (1999).
  • W. R. HARPER, Basic Principles of Fission Reactors, Interscience Publishers Inc., New York (1961).
  • K. O. OTT and W. A. BEZELLA, Nuclear Reactor Statics, American Nuclear Society, La Grange Park, Illinois (1983).
  • J. Y. DORIATH, C. W. MCCALLIEN, E. KIEFHABER, U. WEHMANN, and J. M. RIEUNIER, “ERANOS 1: The Advanced European System of Codes for Reactor Physics Calculations,” Proc. Int. Conf., Karlsruhe, Germany (1993).

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